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Abstract：
Photocatalytic water splitting is a promising and clean way to mimic plant photosynthesis in a sustainable manner. Improvements of the quantum efficiency and optical absorption in the relevant range are necessary steps to approach practicality. Herein, we reported that these issues can be readily addressed when 5-aminotetrazole, a monomer with high nitrogen content, is used for the synthesis of carbon nitride. The molten salt mixture NaCl/KCl is used as a high-temperature solvent to tailor the grain boundary structure and chemistry. Visible light quantum efficiency for H-2 production of 0.65 could be obtained in the presence of K2HPO4 as a double layer modifier. This value is very high, considering that this number depends on light to charge couple conversion, charge localization, as well as a successful oxidation and reduction reaction.
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Source ：
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
ISSN： 1433-7851
Year： 2019
Issue： 11
Volume： 58
Page： 3433-3437
1 2 . 9 5 9
JCR@2019
1 6 . 1 0 0
JCR@2023
ESI Discipline： CHEMISTRY;
ESI HC Threshold：184
JCR Journal Grade：1
CAS Journal Grade：1
Cited Count：
WoS CC Cited Count： 331
SCOPUS Cited Count： 336
ESI Highly Cited Papers on the List： 30 Unfold All
WanFang Cited Count：
Chinese Cited Count：
30 Days PV： 2
Affiliated Colleges：
