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author:

Chen, Qiushui (Chen, Qiushui.) [1] | Wu, Jing (Wu, Jing.) [2] | Ou, Xiangyu (Ou, Xiangyu.) [3] | Huang, Bolong (Huang, Bolong.) [4] | Almutlaq, Jawaher (Almutlaq, Jawaher.) [5] | Zhumekenov, Ayan A. (Zhumekenov, Ayan A..) [6] | Guan, Xinwei (Guan, Xinwei.) [7] | Han, Sanyang (Han, Sanyang.) [8] | Liang, Liangliang (Liang, Liangliang.) [9] | Yi, Zhigao (Yi, Zhigao.) [10] | Li, Juan (Li, Juan.) [11] (Scholars:李娟) | Xie, Xiaoji (Xie, Xiaoji.) [12] | Wang, Yu (Wang, Yu.) [13] | Li, Ying (Li, Ying.) [14] | Fan, Dianyuan (Fan, Dianyuan.) [15] | Teh, Daniel B. L. (Teh, Daniel B. L..) [16] | All, Angelo H. (All, Angelo H..) [17] | Mohammed, Omar F. (Mohammed, Omar F..) [18] | Bakr, Osman M. (Bakr, Osman M..) [19] | Wu, Tom (Wu, Tom.) [20] | Bettinelli, Marco (Bettinelli, Marco.) [21] | Yang, Huanghao (Yang, Huanghao.) [22] (Scholars:杨黄浩) | Huang, Wei (Huang, Wei.) [23] | Liu, Xiaogang (Liu, Xiaogang.) [24]

Indexed by:

Scopus SCIE

Abstract:

The rising demand for radiation detection materials in many applications has led to extensive research on scintillators(1-3). The ability of a scintillator to absorb high-energy (kiloelectronvolt-scale) X-ray photons and convert the absorbed energy into low-energy visible photons is critical for applications in radiation exposure monitoring, security inspection, X-ray astronomy and medical radiography(4,5). However, conventional scintillators are generally synthesized by crystallization at a high temperature and their radioluminescence is difficult to tune across the visible spectrum. Here we describe experimental investigations of a series of all-inorganic perovskite nanocrystals comprising caesium and lead atoms and their response to X-ray irradiation. These nanocrystal scintillators exhibit strong X-ray absorption and intense radioluminescence at visible wavelengths. Unlike bulk inorganic scintillators, these perovskite nanomaterials are solution-processable at a relatively low temperature and can generate X-ray-induced emissions that are easily tunable across the visible spectrum by tailoring the anionic component of colloidal precursors during their synthesis. These features allow the fabrication of flexible and highly sensitive X-ray detectors with a detection limit of 13 nanograys per second, which is about 400 times lower than typical medical imaging doses. We show that these colour-tunable perovskite nanocrystal scintillators can provide a convenient visualization tool for X-ray radiography, as the associated image can be directly recorded by standard digital cameras. We also demonstrate their direct integration with commercial flat-panel imagers and their utility in examining electronic circuit boards under low-dose X-ray illumination.

Keyword:

Community:

  • [ 1 ] [Chen, Qiushui]Natl Univ Singapore, Dept Chem, Singapore, Singapore
  • [ 2 ] [Han, Sanyang]Natl Univ Singapore, Dept Chem, Singapore, Singapore
  • [ 3 ] [Liang, Liangliang]Natl Univ Singapore, Dept Chem, Singapore, Singapore
  • [ 4 ] [Yi, Zhigao]Natl Univ Singapore, Dept Chem, Singapore, Singapore
  • [ 5 ] [Liu, Xiaogang]Natl Univ Singapore, Dept Chem, Singapore, Singapore
  • [ 6 ] [Wu, Jing]China Univ Geosci, Sch Sci, Beijing, Peoples R China
  • [ 7 ] [Ou, Xiangyu]Fuzhou Univ, MOE Key Lab Analyt Sci Food Safety & Biol, Fuzhou, Fujian, Peoples R China
  • [ 8 ] [Li, Juan]Fuzhou Univ, MOE Key Lab Analyt Sci Food Safety & Biol, Fuzhou, Fujian, Peoples R China
  • [ 9 ] [Yang, Huanghao]Fuzhou Univ, MOE Key Lab Analyt Sci Food Safety & Biol, Fuzhou, Fujian, Peoples R China
  • [ 10 ] [Ou, Xiangyu]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Fuzhou, Fujian, Peoples R China
  • [ 11 ] [Li, Juan]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Fuzhou, Fujian, Peoples R China
  • [ 12 ] [Yang, Huanghao]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Fuzhou, Fujian, Peoples R China
  • [ 13 ] [Huang, Bolong]Hong Kong Polytech Univ, Dept Appl Biol & Chem Technol, Hong Kong, Hong Kong, Peoples R China
  • [ 14 ] [Almutlaq, Jawaher]King Abdullah Univ Sci & Technol, Div Phys Sci & Engn, Thuwal, Saudi Arabia
  • [ 15 ] [Zhumekenov, Ayan A.]King Abdullah Univ Sci & Technol, Div Phys Sci & Engn, Thuwal, Saudi Arabia
  • [ 16 ] [Guan, Xinwei]King Abdullah Univ Sci & Technol, Div Phys Sci & Engn, Thuwal, Saudi Arabia
  • [ 17 ] [Mohammed, Omar F.]King Abdullah Univ Sci & Technol, Div Phys Sci & Engn, Thuwal, Saudi Arabia
  • [ 18 ] [Bakr, Osman M.]King Abdullah Univ Sci & Technol, Div Phys Sci & Engn, Thuwal, Saudi Arabia
  • [ 19 ] [Xie, Xiaoji]Nanjing Tech Univ, Inst Adv Mat, Nanjing, Jiangsu, Peoples R China
  • [ 20 ] [Huang, Wei]Nanjing Tech Univ, Inst Adv Mat, Nanjing, Jiangsu, Peoples R China
  • [ 21 ] [Wang, Yu]Shenzhen Univ, SZU NUS Collaborat Innovat Ctr Optoelect Sci & Te, Shenzhen, Peoples R China
  • [ 22 ] [Li, Ying]Shenzhen Univ, SZU NUS Collaborat Innovat Ctr Optoelect Sci & Te, Shenzhen, Peoples R China
  • [ 23 ] [Fan, Dianyuan]Shenzhen Univ, SZU NUS Collaborat Innovat Ctr Optoelect Sci & Te, Shenzhen, Peoples R China
  • [ 24 ] [Liu, Xiaogang]Shenzhen Univ, SZU NUS Collaborat Innovat Ctr Optoelect Sci & Te, Shenzhen, Peoples R China
  • [ 25 ] [Teh, Daniel B. L.]Natl Univ Singapore, Singapore Inst Neurotechnol, Singapore, Singapore
  • [ 26 ] [All, Angelo H.]Natl Univ Singapore, Singapore Inst Neurotechnol, Singapore, Singapore
  • [ 27 ] [All, Angelo H.]Johns Hopkins Sch Med, Dept Biomed Engn, Baltimore, MD USA
  • [ 28 ] [Wu, Tom]Univ New South Wales, Sch Mat Sci & Engn, Sydney, NSW, Australia
  • [ 29 ] [Bettinelli, Marco]Univ Verona, DB, Luminescent Mat Lab, Verona, Italy
  • [ 30 ] [Huang, Wei]Nanjing Univ Posts & Telecommun, Key Lab Organ Elect & Informat Displays, Nanjing, Jiangsu, Peoples R China
  • [ 31 ] [Huang, Wei]Nanjing Univ Posts & Telecommun, Inst Adv Mat, Nanjing, Jiangsu, Peoples R China
  • [ 32 ] [Huang, Wei]Northwestern Polytech Univ, Shaanxi Inst Flexible Elect, Xian, Shaanxi, Peoples R China
  • [ 33 ] [Liu, Xiaogang]NUS Suzhou Res Inst, Ctr Funct Mat, Suzhou, Jiangsu, Peoples R China

Reprint 's Address:

  • 杨黄浩

    [Liu, Xiaogang]Natl Univ Singapore, Dept Chem, Singapore, Singapore;;[Yang, Huanghao]Fuzhou Univ, MOE Key Lab Analyt Sci Food Safety & Biol, Fuzhou, Fujian, Peoples R China;;[Yang, Huanghao]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Fuzhou, Fujian, Peoples R China;;[Huang, Wei]Nanjing Tech Univ, Inst Adv Mat, Nanjing, Jiangsu, Peoples R China;;[Liu, Xiaogang]Shenzhen Univ, SZU NUS Collaborat Innovat Ctr Optoelect Sci & Te, Shenzhen, Peoples R China;;[Huang, Wei]Nanjing Univ Posts & Telecommun, Key Lab Organ Elect & Informat Displays, Nanjing, Jiangsu, Peoples R China;;[Huang, Wei]Nanjing Univ Posts & Telecommun, Inst Adv Mat, Nanjing, Jiangsu, Peoples R China;;[Huang, Wei]Northwestern Polytech Univ, Shaanxi Inst Flexible Elect, Xian, Shaanxi, Peoples R China;;[Liu, Xiaogang]NUS Suzhou Res Inst, Ctr Funct Mat, Suzhou, Jiangsu, Peoples R China

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Source :

NATURE

ISSN: 0028-0836

Year: 2018

Issue: 7721

Volume: 561

Page: 88-93

4 3 . 0 7

JCR@2018

5 0 . 5 0 0

JCR@2023

ESI Discipline: MULTIDISCIPLINARY;

ESI HC Threshold:395

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 1468

SCOPUS Cited Count: 1515

ESI Highly Cited Papers on the List: 32 Unfold All

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30 Days PV: 5

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