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author:

Zheng, Yun (Zheng, Yun.) [1] | Yu, Zihao (Yu, Zihao.) [2] | Ou, Honghui (Ou, Honghui.) [3] | Asiri, Abdullah M. (Asiri, Abdullah M..) [4] | Chen, Yilin (Chen, Yilin.) [5] | Wang, Xinchen (Wang, Xinchen.) [6] (Scholars:王心晨)

Indexed by:

EI Scopus SCIE

Abstract:

Metal-free heterostructure photocatalysts composed of black phosphorus (BP) and polymeric carbon nitride (CN) are successfully synthesized via a one-step liquid exfoliation method assisted by sonication. The combination of BP with CN strengthens the visible-light harvesting ability, facilitates the charge separation in the photocatalytic process, and renders promoted activity of photoinduced molecular oxygen activation, such as superoxide radicals (center dot O-2(-)) evolution and H2O2 production. This work highlights that coupling semiconductors with well-matched band levels provide a flexible route to enhance the performance of photocatalysts for producing reactive oxygen species, and gives ideas for the design of highly active and metal-free materials toward sustainable solar-to-chemical energy conversion and environmental remediation.

Keyword:

black phosphorus carbon nitride molecular oxygen activation photocatalysis reactive oxygen species

Community:

  • [ 1 ] [Zheng, Yun]Fuzhou Univ, Coll Chem, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350002, Fujian, Peoples R China
  • [ 2 ] [Yu, Zihao]Fuzhou Univ, Coll Chem, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350002, Fujian, Peoples R China
  • [ 3 ] [Ou, Honghui]Fuzhou Univ, Coll Chem, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350002, Fujian, Peoples R China
  • [ 4 ] [Wang, Xinchen]Fuzhou Univ, Coll Chem, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350002, Fujian, Peoples R China
  • [ 5 ] [Zheng, Yun]Huaqiao Univ, Coll Mat Sci & Engn, Key Lab Funct Mat Fujian Higher Educ, Xiamen 361021, Peoples R China
  • [ 6 ] [Chen, Yilin]Huaqiao Univ, Coll Mat Sci & Engn, Key Lab Funct Mat Fujian Higher Educ, Xiamen 361021, Peoples R China
  • [ 7 ] [Asiri, Abdullah M.]King Abdulaziz Univ, Fac Sci, Dept Chem, Jeddah 21589, Saudi Arabia

Reprint 's Address:

  • 王心晨

    [Wang, Xinchen]Fuzhou Univ, Coll Chem, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350002, Fujian, Peoples R China

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Source :

ADVANCED FUNCTIONAL MATERIALS

ISSN: 1616-301X

Year: 2018

Issue: 10

Volume: 28

1 5 . 6 2 1

JCR@2018

1 8 . 5 0 0

JCR@2023

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:284

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 398

SCOPUS Cited Count: 416

ESI Highly Cited Papers on the List: 36 Unfold All

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  • 2019-9
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WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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