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author:

Qin, Na (Qin, Na.) [1] | Xiong, Jinhua (Xiong, Jinhua.) [2] | Liang, Ruowen (Liang, Ruowen.) [3] | Liu, Yuhao (Liu, Yuhao.) [4] | Zhang, Shiying (Zhang, Shiying.) [5] | Li, Yanhua (Li, Yanhua.) [6] | Li, Zhaohui (Li, Zhaohui.) [7] (Scholars:李朝晖) | Wu, Ling (Wu, Ling.) [8] (Scholars:吴棱)

Indexed by:

EI Scopus SCIE

Abstract:

MoS2/CdS-TiO2 nanofibers have been successfully prepared by an electrospinning mediated photodeposition method for improving the interfacial contact between MoS2 and CdS-TiO2 nanofibers. The structural features, morphologies, and photo-absorption performances of the as-prepared samples were investigated in detail. The photocatalytic activity of a typical sample 1%MoS2/CdS-TiO2(60) nanofibers for H-2 evolution under visible light irradiation exhibits 3.0 and 4.0 times higher than that of 1%MoS2/CdSP25(60) and 1%Pt/CdS-TiO2(60), respectively. Based on the above results, it reveals that one dimensional TiO2 nanofibers can serve as excellent substrates for improving the dispersion of CdS and MoS2. Moreover, the intimate interaction among MoS2, CdS and TiO2 may be suggested by HRTEM images and elements mapping patterns. Further photoelectrochemical analyses show that the, effective separation of photogenerated carriers can be markedly accelerated. Finally, a tentative photocatalytic reaction mechanism has also been investigated. This work demonstrates that the method of combining electrospinning and photodeposition is feasible for the preparation of an effective MoS2/CdS-TiO2 nanofibers composite photocatalyst. (C) 2016 Elsevier B.V. All rights reserved.

Keyword:

Electrospinning Interfacial contact MoS2/CdS-TiO2 nanofibers Photocatalytic H-2 evolution Photodeposition

Community:

  • [ 1 ] [Qin, Na]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350002, Peoples R China
  • [ 2 ] [Xiong, Jinhua]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350002, Peoples R China
  • [ 3 ] [Liang, Ruowen]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350002, Peoples R China
  • [ 4 ] [Liu, Yuhao]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350002, Peoples R China
  • [ 5 ] [Li, Zhaohui]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350002, Peoples R China
  • [ 6 ] [Wu, Ling]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350002, Peoples R China
  • [ 7 ] [Zhang, Shiying]Changsha Univ, Hunan Prov Key Lab Appl Environm Photocatalysis, Changsha 410022, Hunan, Peoples R China
  • [ 8 ] [Li, Yanhua]Changsha Univ, Hunan Prov Key Lab Appl Environm Photocatalysis, Changsha 410022, Hunan, Peoples R China

Reprint 's Address:

  • 李朝晖 吴棱

    [Li, Zhaohui]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350002, Peoples R China;;[Wu, Ling]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350002, Peoples R China

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Source :

APPLIED CATALYSIS B-ENVIRONMENTAL

ISSN: 0926-3373

Year: 2017

Volume: 202

Page: 374-380

1 1 . 6 9 8

JCR@2017

2 0 . 3 0 0

JCR@2023

ESI Discipline: CHEMISTRY;

ESI HC Threshold:226

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 190

SCOPUS Cited Count: 199

ESI Highly Cited Papers on the List: 18 Unfold All

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WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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