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author:

Zhang, Guigang (Zhang, Guigang.) [1] (Scholars:张贵刚) | Lan, Zhi-An (Lan, Zhi-An.) [2] (Scholars:蓝志安) | Lin, Lihua (Lin, Lihua.) [3] | Lin, Sen (Lin, Sen.) [4] (Scholars:林森) | Wang, Xinchen (Wang, Xinchen.) [5] (Scholars:王心晨)

Indexed by:

EI Scopus SCIE

Abstract:

We report the direct splitting of pure water by light-excited graphitic carbon nitride (g-C3N4) modified with Pt, PtOx, and CoOx as redox cocatalysts, while pure g-C3N4 is virtually inactive for overall water splitting by photocatalysis. The novelty is in the selective creation of both H-2 and O-2 cocatalysts on surface active sites of g-C3N4 via photodeposition triggering the splitting of water for the simultaneous evolution of H-2 and O-2 gases in a stoichiometric ratio of 2 : 1, irradiated with light, without using any sacrificial reagents. The photocatalyst was stable for 510 hours of reaction.

Keyword:

Community:

  • [ 1 ] [Zhang, Guigang]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Coll Chem, Fuzhou 350002, Peoples R China
  • [ 2 ] [Lan, Zhi-An]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Coll Chem, Fuzhou 350002, Peoples R China
  • [ 3 ] [Lin, Lihua]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Coll Chem, Fuzhou 350002, Peoples R China
  • [ 4 ] [Lin, Sen]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Coll Chem, Fuzhou 350002, Peoples R China
  • [ 5 ] [Wang, Xinchen]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Coll Chem, Fuzhou 350002, Peoples R China

Reprint 's Address:

  • 王心晨

    [Wang, Xinchen]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Coll Chem, Fuzhou 350002, Peoples R China

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Source :

CHEMICAL SCIENCE

ISSN: 2041-6520

Year: 2016

Issue: 5

Volume: 7

Page: 3062-3066

8 . 6 6 8

JCR@2016

7 . 6 0 0

JCR@2023

ESI Discipline: CHEMISTRY;

ESI HC Threshold:235

JCR Journal Grade:1

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count: 828

SCOPUS Cited Count: 871

ESI Highly Cited Papers on the List: 44 Unfold All

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Chinese Cited Count:

30 Days PV: 0

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