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Abstract:
Here, we show for the first time that the photocatalytic activity of covalent triazine-based frameworks (CTFs) can be efficiently improved using a facile sulfur-doping approach. The sulfur-doped CTFs show superior photocatalytic activity and stability in hydrogen evolution from water under visible light irradiation over pristine CTFs and g-C3N4. The significantly improved catalytic efficiency was attributed to sulfur-doping in the frameworks, which results in enhanced adsorption of visible light, reduced recombination of free charge carriers, and rapid separation and transportation of photogenerated electronholes.
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JOURNAL OF MATERIALS CHEMISTRY A
ISSN: 2050-7488
Year: 2016
Issue: 32
Volume: 4
Page: 12402-12406
8 . 8 6 7
JCR@2016
1 0 . 8 0 0
JCR@2023
ESI Discipline: MATERIALS SCIENCE;
ESI HC Threshold:324
JCR Journal Grade:1
CAS Journal Grade:1
Cited Count:
WoS CC Cited Count: 202
SCOPUS Cited Count: 195
ESI Highly Cited Papers on the List: 0 Unfold All
WanFang Cited Count:
Chinese Cited Count:
30 Days PV: 3