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Abstract：
The combination of cobalt redox catalysis and carbon nitride photocatalysis to construct a cascade photoreaction system has been developed for the deoxygenative reduction of CO2 to CO with visible light. The graphitic carbon nitride has been demonstrated to function both as a capture/activation substrate of CO2 and a photocatalyst, whereas the introduced cobalt species act as reductive and oxidative promoters to accelerate charge-carrier separation and transfer kinetics. This hybrid photosystem contains inexpensive substances that synergetically catalyze CO2-to-CO conversion at mild conditions, with a high stability of catalysts. The optimization in the surface and texture structures as well as reaction conditions has been demonstrated. The results represent an important step toward artificial photosynthesis by using cost-acceptable materials.
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ACS SUSTAINABLE CHEMISTRY & ENGINEERING
ISSN： 2168-0485
Year： 2014
Issue： 3
Volume： 2
Page： 353-358
4 . 6 4 2
JCR@2014
7 . 1 0 0
JCR@2023
ESI Discipline： CHEMISTRY;
ESI HC Threshold：268
JCR Journal Grade：1
CAS Journal Grade：2
Cited Count：
WoS CC Cited Count： 361
SCOPUS Cited Count： 373
ESI Highly Cited Papers on the List： 36 Unfold All
WanFang Cited Count：
Chinese Cited Count：
30 Days PV： 2
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