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author:

Li, Wenjuan (Li, Wenjuan.) [1] | Li, Danzhen (Li, Danzhen.) [2] (Scholars:李旦振) | Wang, Jinxiu (Wang, Jinxiu.) [3] | Shao, Yu (Shao, Yu.) [4] (Scholars:邵宇) | You, Jinmao (You, Jinmao.) [5] | Teng, Fei (Teng, Fei.) [6]

Indexed by:

EI Scopus SCIE

Abstract:

The systematic clarification of the photocatalytic process in different kinds of systems is significantly instructive to recognize the photocatalytic mechanism and design novel efficient photocatalysts. The types of the active species (such as (OH)-O-center dot and O-2(center dot-)) generated in the photocatalytic process are complicated and their roles playing in the photocatalysis remain obscure and controversial. Aimed at these problems, the active species in the degradation process of methyl orange (MO) were investigated by using TiO2 and ZnO photocatalysts. Various surface analysis techniques (NMR, ESR, photoluminescence technique, etc.) were used to study their mechanisms in the degradation of MO under UV light irradiation. As a result, it was found that in TiO2 system, (OH)-O-center dot was generated by photo-generated holes; while in ZnO system, (OH)-O-center dot was generated by photo-generated holes and O-2(center dot-). The larger numbers of the active species and their incessant sources in ZnO system contributed to the better activity. The conclusions were first found in the investigation of the active species between the two catalysts and would provide certain theoretical guidance in seeking the new pathway to increase the concentration of the active species and the photocatalytic activity. (C) 2013 Elsevier B.V. All rights reserved.

Keyword:

Active species Mechanism (OH)-O-center dot Oxygen species Photocatalysis

Community:

  • [ 1 ] [Li, Wenjuan]Qufu Normal Univ, Shandong Prov Key Lab Life Organ Anal, Qufu 273165, Peoples R China
  • [ 2 ] [You, Jinmao]Qufu Normal Univ, Shandong Prov Key Lab Life Organ Anal, Qufu 273165, Peoples R China
  • [ 3 ] [Li, Wenjuan]Fuzhou Univ, Fujian Prov Key Lab Photocatalysis, State Key Lab Breeding Base, Fuzhou 350002, Peoples R China
  • [ 4 ] [Li, Danzhen]Fuzhou Univ, Fujian Prov Key Lab Photocatalysis, State Key Lab Breeding Base, Fuzhou 350002, Peoples R China
  • [ 5 ] [Wang, Jinxiu]Fuzhou Univ, Fujian Prov Key Lab Photocatalysis, State Key Lab Breeding Base, Fuzhou 350002, Peoples R China
  • [ 6 ] [Shao, Yu]Fuzhou Univ, Fujian Prov Key Lab Photocatalysis, State Key Lab Breeding Base, Fuzhou 350002, Peoples R China
  • [ 7 ] [Li, Wenjuan]Nanjing Univ Informat Sci & Engn, Sch Environm Sci & Engn, Jiangsu Key Lab Atmospher Environm Monitoring & P, Nanjing 210044, Jiangsu, Peoples R China
  • [ 8 ] [Teng, Fei]Nanjing Univ Informat Sci & Engn, Sch Environm Sci & Engn, Jiangsu Key Lab Atmospher Environm Monitoring & P, Nanjing 210044, Jiangsu, Peoples R China

Reprint 's Address:

  • 李旦振

    [Li, Danzhen]Qufu Normal Univ, Shandong Prov Key Lab Life Organ Anal, Qufu 273165, Peoples R China

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Source :

JOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL

ISSN: 1381-1169

Year: 2013

Volume: 380

Page: 10-17

3 . 6 7 9

JCR@2013

5 . 0 0 8

JCR@2018

JCR Journal Grade:2

CAS Journal Grade:3

Cited Count:

WoS CC Cited Count: 59

SCOPUS Cited Count: 62

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 3

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