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author:

Yang, Yu (Yang, Yu.) [1] | Ji, Tao (Ji, Tao.) [2] | Su, Wenyue (Su, Wenyue.) [3] | Yang, Bin (Yang, Bin.) [4] | Zhang, Yong (Zhang, Yong.) [5] | Yang, Zhengxian (Yang, Zhengxian.) [6]

Indexed by:

EI

Abstract:

The combination of photocatalyst with cementitious materials for air pollution abatement and self-cleaning has gained considerable attention. However, the most popularly used photocatalytic cementitious composites based on TiO2 achieve the purification function under ultraviolet sunlight, significantly impeding a broader application of photocatalytic cementitious composites. Here, the photocatalytic cementitious composites were prepared by incorporating g-C3N4 nanosheets (CNNs) in Portland cement. With the increase of CNNs content, the photocatalytic NOx abatement and self-cleaning performance was notably improved, while the micro-hardness of cementitious composites increased first and then decreased. Among the three mixing dosages (0.5%, 1% and 2% by weight of cement), the cementitious composite admixed with 2% CNNs showed the highest photocatalytic NOx abatement efficiency of 227.3 μmol m−2 h−1, and could degrade the rhodamine B within 40 min under visible light. Additionally, its microscopic hardness was 5.4% higher than the one without CNNs, suggesting that a moderate amount of CNNs (below 2%) in cementitious composites was effective in achieving an improved photocatalytic depollution performance. © 2019 Elsevier Ltd

Keyword:

Air cleaners Cleaning Hydration Light Microhardness Nanosheets Nitrogen oxides Oxide minerals Photocatalytic activity Pollution control Portland cement Rhodamine B Titanium dioxide

Community:

  • [ 1 ] [Yang, Yu]Fujian Provincial University Research Center for Advanced Civil Engineering Materials, Fuzhou University, Fuzhou; 350116, China
  • [ 2 ] [Yang, Yu]College of Civil Engineering, Fuzhou University, Fuzhou; 350116, China
  • [ 3 ] [Ji, Tao]College of Civil Engineering, Fuzhou University, Fuzhou; 350116, China
  • [ 4 ] [Su, Wenyue]State Key Laboratory of Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou; 350116, China
  • [ 5 ] [Yang, Bin]Chengdu Design & Research Institute of Building Materials Industry Co., Ltd, Chengdu; 610051, China
  • [ 6 ] [Zhang, Yong]Fujian Provincial University Research Center for Advanced Civil Engineering Materials, Fuzhou University, Fuzhou; 350116, China
  • [ 7 ] [Zhang, Yong]Microlab, Section of Materials and Environment, Faculty of Civil Engineering and Geosciences, Delft University of Technology, Stevinweg 1, CN Delft; 2628, Netherlands
  • [ 8 ] [Yang, Zhengxian]Fujian Provincial University Research Center for Advanced Civil Engineering Materials, Fuzhou University, Fuzhou; 350116, China
  • [ 9 ] [Yang, Zhengxian]College of Civil Engineering, Fuzhou University, Fuzhou; 350116, China
  • [ 10 ] [Yang, Zhengxian]Department of Civil & Environmental Engineering, Washington State University, Pullman; WA; 99164-2910, United States

Reprint 's Address:

  • [yang, zhengxian]college of civil engineering, fuzhou university, fuzhou; 350116, china;;[yang, zhengxian]department of civil & environmental engineering, washington state university, pullman; wa; 99164-2910, united states;;[yang, zhengxian]fujian provincial university research center for advanced civil engineering materials, fuzhou university, fuzhou; 350116, china

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Source :

Construction and Building Materials

ISSN: 0950-0618

Year: 2019

Volume: 225

Page: 120-131

4 . 4 1 9

JCR@2019

7 . 4 0 0

JCR@2023

ESI HC Threshold:236

JCR Journal Grade:1

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 30

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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