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author:

Tan, Li (Tan, Li.) [1] | Zhang, Peipei (Zhang, Peipei.) [2] | Cui, Yu (Cui, Yu.) [3] | Suzuki, Yuichi (Suzuki, Yuichi.) [4] | Li, Hangjie (Li, Hangjie.) [5] | Guo, Lisheng (Guo, Lisheng.) [6] | Yang, Guohui (Yang, Guohui.) [7] | Tsubaki, Noritatsu (Tsubaki, Noritatsu.) [8]

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EI

Abstract:

We evaluate the direct CO2 conversion to light olefins reaction via a hybrid catalyst of In2O3/ZrO2 metallic oxide and zeolite SAPO34 components. On this catalyst, it can realize producing high light olefins selectivity of 77.59% via a direct tandem catalysis process, that is, the formed methanol on the oxygen vacancies surface of In2O3/ZrO2 in the first step will continue passing through the SAPO34 zeolite channel, where it is changed into light olefins simultaneously. Even there are many studies focused on this tandem catalysis reaction via bi-functional catalyst in recent years, however, to reduce the poisonous byproduct CO is still in a big challenge. In this reaction, large amounts of poisonous CO will be easily formed from reverse water gas shift reaction. Therefore, in our research, by optimizing the reaction, the catalyst can suppress the undesirable CO formation obviously. It shows good potential leading to scale-up cause of the outstanding reaction performance and its friendly-environment properties. © 2019 Elsevier B.V.

Keyword:

Carbon dioxide Catalysis Catalyst selectivity Chemical shift Cobalt Hydrogenation Indium compounds Light olefins Metals Water gas shift Zeolites

Community:

  • [ 1 ] [Tan, Li]Institute of In Situ, Operando Studies of Catalysis and College of Chemistry, Fuzhou University, Fuzhou; 350108, China
  • [ 2 ] [Tan, Li]Department of Applied Chemistry, School of Engineering, University of Toyama, Gofuku 3190, Toyama; 930-8555, Japan
  • [ 3 ] [Zhang, Peipei]Department of Applied Chemistry, School of Engineering, University of Toyama, Gofuku 3190, Toyama; 930-8555, Japan
  • [ 4 ] [Cui, Yu]Department of Applied Chemistry, School of Engineering, University of Toyama, Gofuku 3190, Toyama; 930-8555, Japan
  • [ 5 ] [Suzuki, Yuichi]Department of Applied Chemistry, School of Engineering, University of Toyama, Gofuku 3190, Toyama; 930-8555, Japan
  • [ 6 ] [Li, Hangjie]Department of Applied Chemistry, School of Engineering, University of Toyama, Gofuku 3190, Toyama; 930-8555, Japan
  • [ 7 ] [Guo, Lisheng]Department of Applied Chemistry, School of Engineering, University of Toyama, Gofuku 3190, Toyama; 930-8555, Japan
  • [ 8 ] [Yang, Guohui]Department of Applied Chemistry, School of Engineering, University of Toyama, Gofuku 3190, Toyama; 930-8555, Japan
  • [ 9 ] [Yang, Guohui]State Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of Sciences, Taiyuan; 030001, China
  • [ 10 ] [Tsubaki, Noritatsu]Department of Applied Chemistry, School of Engineering, University of Toyama, Gofuku 3190, Toyama; 930-8555, Japan

Reprint 's Address:

  • [yang, guohui]department of applied chemistry, school of engineering, university of toyama, gofuku 3190, toyama; 930-8555, japan;;[yang, guohui]state key laboratory of coal conversion, institute of coal chemistry, chinese academy of sciences, taiyuan; 030001, china

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Source :

Fuel Processing Technology

ISSN: 0378-3820

Year: 2019

Volume: 196

4 . 9 8 2

JCR@2019

7 . 2 0 0

JCR@2023

ESI HC Threshold:184

JCR Journal Grade:1

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count: 0

SCOPUS Cited Count: 76

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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