• Complex
  • Title
  • Keyword
  • Abstract
  • Scholars
  • Journal
  • ISSN
  • Conference
成果搜索

author:

Lin, Lihua (Lin, Lihua.) [1] | Ou, Honghui (Ou, Honghui.) [2] | Zhang, Yongfan (Zhang, Yongfan.) [3] | Wang, Xinchen (Wang, Xinchen.) [4]

Indexed by:

EI

Abstract:

Graphitic carbon nitride (g-CN) is an emerging metal-free photocatalyst for solar energy conversion via water splitting and CO2 fixation. Herein, we used preheated melamine as a starting material in combination with the salt melt method to synthesize a crystalline tri-s-triazine-based g-CN. The as-obtained sample exhibited high stability and photocatalytic activity toward hydrogen and oxygen production from water splitting. In addition, by adding phosphate to mimic natural photosynthetic environment, the apparent quantum yield (AQY) for the hydrogen production reached 50.7% at 405 nm, which is the highest value ever reported for conjugated carbon nitride polymers in hydrogen evolution photocatalysis. The results of this study demonstrate that crystalline covalent tri-s-triazine frameworks hold great promise for solar energy applications. © 2016 American Chemical Society.

Keyword:

Carbon nitride Conjugated polymers Crystalline materials Energy conversion Hydrogen production Natural polymers Nitrides Photocatalysis Photocatalytic activity Polyols Solar energy

Community:

  • [ 1 ] [Lin, Lihua]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350002, China
  • [ 2 ] [Ou, Honghui]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350002, China
  • [ 3 ] [Zhang, Yongfan]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350002, China
  • [ 4 ] [Wang, Xinchen]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350002, China

Reprint 's Address:

  • [wang, xinchen]state key laboratory of photocatalysis on energy and environment, college of chemistry, fuzhou university, fuzhou; 350002, china

Show more details

Related Keywords:

Source :

ACS Catalysis

Year: 2016

Issue: 6

Volume: 6

Page: 3921-3931

1 0 . 6 1 4

JCR@2016

1 1 . 7 0 0

JCR@2023

ESI HC Threshold:235

JCR Journal Grade:1

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 828

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 4

Affiliated Colleges:

Online/Total:367/10023176
Address:FZU Library(No.2 Xuyuan Road, Fuzhou, Fujian, PRC Post Code:350116) Contact Us:0591-22865326
Copyright:FZU Library Technical Support:Beijing Aegean Software Co., Ltd. 闽ICP备05005463号-1