Physical Properties of a Promising Nonlinear Optical Crystal K3Ba3Li2Al4B6O20F - Details

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Abstract：

Beryllium-free　nonlinear　optical　(NLO)　crystal　K3Ba3Li2Al4B6O20F　(KBLABF)　is　a　newly　reported　promising　candidate　in　the　generation　of　the　significant　UV　coherent　light.　A　17　×　12　×　8　mm3　bulk　single　crystal　is　successfully　grown　with　an　optimized　flux　molar　ratio.　The　crystal　specific　heat　increases　from　0.65　J·g-1·°C-1　to　0.96　J·g-1·°C-1　with　the　increasing　temperature.　Meanwhile,　the　a-direction　thermal　conductivity　of　KBLABF　is　1.11　W·m-1·K-1　at　25　°C,　which　is　also　equivalent　to　that　of　the　famous　NLO　crystal　β-BaB2O4　(1.25　W·m-1·K-1).　The　KBLABF　crystal　has　moderate　Vickers　hardness　along　the　a-axis　and　c-axis　(165.1　HV0.1　and　257.7　HV0.1,　respectively),　which　indicates　it　is　easy　to　be　cut　and　polished.　Remarkably,　the　laser　damage　threshold　of　KBLABF　is　3.32　GW·cm-2　(1064　nm,　8　ns),　which　even　exceeds　those　of　some　famous　commercial　NLO　crystals.　This　result　demonstrates　that　KBLABF　is　suitable　for　high-power　NLO　applications.　This　work　will　establish　the　foundation　for　the　future　NLO　applications　of　the　KBLABF　crystal.　Copyright　©　2018　American　Chemical　Society.

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[ 1 ] [Zhao, B.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, Fujian 350002, China
[ 2 ] [Zhao, B.]College of Chemistry, Fuzhou University, Fuzhou, 350116, China
[ 3 ] [Li, B.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, Fujian 350002, China
[ 4 ] [Zhao, S.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, Fujian 350002, China
[ 5 ] [Liu, X.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, Fujian 350002, China
[ 6 ] [Wu, Z.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, Fujian 350002, China
[ 7 ] [Shen, Y.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, Fujian 350002, China
[ 8 ] [Li, X.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, Fujian 350002, China
[ 9 ] [Ding, Q.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, Fujian 350002, China
[ 10 ] [Ji, C.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, Fujian 350002, China
[ 11 ] [Luo, J.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, Fujian 350002, China

Reprint 's Address：

[Zhao, S.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of SciencesChina

Email：

zhaosangen@fjirsm.ac.cn

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Crystal Growth and Design

ISSN： 1528-7483

Year： 2018

Issue： 12

Volume： 18

Page： 7368-7372

4 . 1 5 3

JCR@2018

3 . 2 0 0

JCR@2023

ESI HC Threshold：209

JCR Journal Grade：1

CAS Journal Grade：2

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ESI Highly Cited Papers on the List： 0 Unfold All

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30 Days PV： 0

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