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author:

Fan, G. (Fan, G..) [1] | Zhan, J. (Zhan, J..) [2] | Luo, J. (Luo, J..) [3] | Lin, J. (Lin, J..) [4] | Qu, F. (Qu, F..) [5] | Du, B. (Du, B..) [6] | You, Y. (You, Y..) [7] | Yan, Z. (Yan, Z..) [8]

Indexed by:

Scopus

Abstract:

In this work, a novel Ag/AgCl@g-C3N4@UIO-66(NH2) heterojunction was constructed for photocatalytic inactivation of Microcystis aeruginosa (M. aeruginosa) under visible light. The photocatalyst was synthesized by a facile method and characterized by XRD, SEM, TEM, BET, XPS, FT−IR, UV–vis DRS, PL and EIS. The nanocomposite can not only provide lots of active sites, but also improve capacities to utilize visible-light energy and effectively transfer charge carriers, thus enhancing removal efficiencies of cyanobacteria (99.9% chlorophyll a was degraded within 180 min). Various factors in photodegradation of chlorophyll a were studied. Besides, changes on cellular morphologies, membrane permeability, physiological activities of M. aeruginosa during photocatalysis were investigated. Moreover, the cycle test indicated that Ag/AgCl@g-C3N4@UIO-66(NH2) exhibits excellent reusability and photocatalytic stability. Finally, a possible mechanism of M. aeruginosa inactivation was proposed. In a word, Ag/AgCl@g-C3N4@UIO-66(NH2) can efficiently inactivate cyanobacteria under visible light, thus providing useful references for further removal of harmful algae in real water bodies. © 2020 Elsevier B.V.

Keyword:

Ag/AgCl@g-C3N4@UIO-66(NH2); G-C3N4@Mof; Heterojunction; Microcystis aeruginosa; Visible light

Community:

  • [ 1 ] [Fan, G.]College of Civil Engineering, Fuzhou University, Fujian, 350116, China
  • [ 2 ] [Fan, G.]State Key Laboratory of Photocatalysis on Energy and Environment, Fuzhou University, Fujian, 350002, China
  • [ 3 ] [Fan, G.]Fujian Provincial Key Laboratory of Electrochemical Energy Storage Materials, Fuzhou University, Fujian, 350002, China
  • [ 4 ] [Zhan, J.]College of Civil Engineering, Fuzhou University, Fujian, 350116, China
  • [ 5 ] [Luo, J.]Fujian Jinhuang Environmental Sci-Tech Co. Ltd, Fujian, 350002, China
  • [ 6 ] [Lin, J.]Fujian Provincial Engineering Research Center of Rural Waste Recycling Technology, School of Environment and Resources, Fuzhou University, Fuzhou, 350116, China
  • [ 7 ] [Qu, F.]Key Laboratory for Water Quality and Conservation of the Pearl River Delta, Guangzhou University, Guangzhou, 510006, China
  • [ 8 ] [Du, B.]College of Civil Engineering, Fuzhou University, Fujian, 350116, China
  • [ 9 ] [You, Y.]College of Civil Engineering, Fuzhou University, Fujian, 350116, China
  • [ 10 ] [Yan, Z.]College of Civil Engineering, Fuzhou University, Fujian, 350116, China
  • [ 11 ] [Yan, Z.]State Key Laboratory of Photocatalysis on Energy and Environment, Fuzhou University, Fujian, 350002, China
  • [ 12 ] [Yan, Z.]Fujian Provincial Key Laboratory of Electrochemical Energy Storage Materials, Fuzhou University, Fujian, 350002, China

Reprint 's Address:

  • [Yan, Z.]College of Civil Engineering, Fuzhou UniversityChina

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Source :

Journal of Hazardous Materials

ISSN: 0304-3894

Year: 2021

Volume: 404

1 4 . 2 2 4

JCR@2021

1 2 . 2 0 0

JCR@2023

ESI HC Threshold:105

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 145

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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