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author:

Yu, J. (Yu, J..) [1] | Lei, J. (Lei, J..) [2] | Wang, L. (Wang, L..) [3] | Guillard, C. (Guillard, C..) [4] | Zhang, J. (Zhang, J..) [5] | Liu, Y. (Liu, Y..) [6] | Anpo, M. (Anpo, M..) [7]

Indexed by:

Scopus

Abstract:

The utilization of TiO2-based photocatalysts for an efficient removal of dye pollutants is limited due to their low surface area, high recombination rate of the photo-generated electrons and holes and an insufficient absorption of sunlight with only 3–4% use of solar energy. Based on this background, we have successfully fabricated a carbon nitride quantum dots (CNQDs)-modified mesoporous TiO2–SiO2 (Me-TSCN) via a simple calcination method since the mesoporous structure is expected to induce a great increase in the specific surface area by carbon nitride quantum dots, being favorable for the adsorption of the reactant molecules and the mass transfer of the reaction products. Furthermore, such CNQD modification facilitates the separation of photo-generated electrons and holes. As a result, the composite's modification with structural design could significantly improve the photocatalytic activity of TiO2-based catalysts, achieving outstanding photocatalytic activity in the degradation of dye pollutants such as rhodamine B. © 2019, Springer Nature B.V.

Keyword:

Dye degradation; Mesopores; Quantum dots

Community:

  • [ 1 ] [Yu, J.]State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control on Chemical Process, School of Resources and Environmental Engineering, East China University of Science and Technology, 130 Meilong Road, Shanghai, 200237, China
  • [ 2 ] [Lei, J.]State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control on Chemical Process, School of Resources and Environmental Engineering, East China University of Science and Technology, 130 Meilong Road, Shanghai, 200237, China
  • [ 3 ] [Lei, J.]Shanghai Institute of Pollution Control and Ecological Security, Shanghai, 200092, China
  • [ 4 ] [Wang, L.]Key Lab for Advanced Materials and Institute of Fine Chemicals, East China University of Science and Technology, 130 Meilong Road, Shanghai, 200237, China
  • [ 5 ] [Guillard, C.]University of Lyon, Institute of Researches on Catalysis and Environment in Lyon (IRCELYON) CNRS, Université Claude Bernard Lyon 1, Villeurbanne, 69626, France
  • [ 6 ] [Zhang, J.]Key Lab for Advanced Materials and Institute of Fine Chemicals, East China University of Science and Technology, 130 Meilong Road, Shanghai, 200237, China
  • [ 7 ] [Liu, Y.]State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control on Chemical Process, School of Resources and Environmental Engineering, East China University of Science and Technology, 130 Meilong Road, Shanghai, 200237, China
  • [ 8 ] [Liu, Y.]Shanghai Institute of Pollution Control and Ecological Security, Shanghai, 200092, China
  • [ 9 ] [Anpo, M.]State Key Laboratory of Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou, Fujian 350116, China
  • [ 10 ] [Anpo, M.]Department of Applied Chemistry, Osaka Prefecture University, Sakai, Osaka 598-8531, Japan

Reprint 's Address:

  • [Liu, Y.]State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control on Chemical Process, School of Resources and Environmental Engineering, East China University of Science and Technology, 130 Meilong Road, China

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Source :

Research on Chemical Intermediates

ISSN: 0922-6168

Year: 2019

Issue: 8

Volume: 45

Page: 4237-4247

2 . 2 6 2

JCR@2019

2 . 8 0 0

JCR@2023

ESI HC Threshold:184

JCR Journal Grade:3

CAS Journal Grade:4

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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