Interfacial engineering of Ru-S-Sb/antimonene electrocatalysts for highly efficient electrolytic hydrogen generation in neutral electrolyte - Details

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The　development　of　high-kinetic　catalysts　for　the　hydrogen　evolution　reaction　(HER)　in　a　neutral　electrolyte　is　of　great　importance　but　unfortunately　remains　a　challenge　so　far.　Herein,　we　report　hybrids　with　abundant　Ru-S-Sb　bonds　and　engineered　ultrathin　antimonene　(Ru-S-Sb/antimonene)　as　highly　kinetic,　active,　stable　electrocatalysts　for　the　HER　in　an　aqueous　neutral　electrolyte.　Experiments　and　density　functional　theory　(DFT)　calculations　reveal　that　Ru-S-Sb　bonds　coupling　with　antimonene　synergistically　work　to　promote　HER　activity.　The　present　study　brings　us　one　step　closer　to　understand　the　structure-composition-property　relationships　and　practical　electrolytic　H2　production.　This　journal　is　©　2019　The　Royal　Society　of　Chemistry.

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[ 1 ] [Li, Y.]Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou, 310027, China
[ 2 ] [Chen, J.]CAS Key Lab. of Des. and Assembly of Funct. Nanostructures and Fujian Prov. Key Lab. of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou Fujian, 350002, China
[ 3 ] [Huang, J.]CAS Key Lab. of Des. and Assembly of Funct. Nanostructures and Fujian Prov. Key Lab. of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou Fujian, 350002, China
[ 4 ] [Hou, Y.]Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou, 310027, China
[ 5 ] [Lei, L.]Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou, 310027, China
[ 6 ] [Lin, W.]MOE Key Laboratory for Analytical Science of Food Safety and Biology, State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350116, China
[ 7 ] [Lian, Y.]MOE Key Laboratory for Analytical Science of Food Safety and Biology, State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350116, China
[ 8 ] [Zhonghua, X.]Beijing Advanced Innovation Center for Soft Matter Science and Engineering, State Key Laboratory of Organic-Inorganic Composites, College of Chemical Engineering, College of Energy, Beijing University of Chemical Technology, Beijing, 100029, China
[ 9 ] [Yang, H.-H.]MOE Key Laboratory for Analytical Science of Food Safety and Biology, State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350116, China
[ 10 ] [Wen, Z.]CAS Key Lab. of Des. and Assembly of Funct. Nanostructures and Fujian Prov. Key Lab. of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou Fujian, 350002, China

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Chemical Communications

ISSN： 1359-7345

Year： 2019

Issue： 73

Volume： 55

Page： 10884-10887

5 . 9 9 6

JCR@2019

4 . 3 0 0

JCR@2023

ESI HC Threshold：184

JCR Journal Grade：1

CAS Journal Grade：2

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SCOPUS Cited Count： 26

ESI Highly Cited Papers on the List： 0 Unfold All

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30 Days PV： 0

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