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author:

Sun, W. (Sun, W..) [1] | Cheng, H. (Cheng, H..) [2] | Lin, N. (Lin, N..) [3] | Lu, Y. (Lu, Y..) [4] | Chen, L. (Chen, L..) [5] | Zhao, Y. (Zhao, Y..) [6] | Francis, P.S. (Francis, P.S..) [7] | Zhuang, N. (Zhuang, N..) [8] | Zheng, Y. (Zheng, Y..) [9]

Indexed by:

Scopus

Abstract:

Carbon nitride, regarded as a promising, environmentally friendly and sustainable photocatalyst for solar hydrogen generation, has shown a gradual improvement of photocatalytic activity with an apparent quantum yield up to 60%. However, it is still challenging to achieve flexible, efficient and scalable carbon nitride solar hydrogen evolution devices, limiting its practical application. Herein we report a visible-light-driven double-side hydrogen evolution nanopaper that is highly porous, crystalline and chemically stable. The nanopaper was fabricated via vacuum filtration of electrostatically self-assembled carbon nitride and nanocellulose. This nanopaper shows excellent mechanical properties with tensile strength of 18.5 MPa and Young's modulus of 414 MPa, a high hydrogen evolution rate of 3.9 mmol g−1 h−1 (corresponding to 6.5 μmol cm−2 h−1), and remarkable photostability over 32-h photocatalytic tests. © 2019 Elsevier B.V.

Keyword:

Cellulose nanofibers; Free-standing thin films; g-C3N4; Nanopapers; Solar hydrogen evolution

Community:

  • [ 1 ] [Sun, W.]College of Chemistry, Fuzhou University, Fuzhou, 350116, China
  • [ 2 ] [Cheng, H.]College of Chemistry, Fuzhou University, Fuzhou, 350116, China
  • [ 3 ] [Lin, N.]College of Chemistry, Fuzhou University, Fuzhou, 350116, China
  • [ 4 ] [Lu, Y.]College of Chemistry, Fuzhou University, Fuzhou, 350116, China
  • [ 5 ] [Chen, L.]College of Chemistry, Fuzhou University, Fuzhou, 350116, China
  • [ 6 ] [Zhao, Y.]College of Chemistry, Fuzhou University, Fuzhou, 350116, China
  • [ 7 ] [Francis, P.S.]School of Life and Environmental Sciences, Faculty of Science, Engineering and Built Environment, Deakin University, Waurn PondsVictoria 3216, Australia
  • [ 8 ] [Zhuang, N.]College of Chemistry, Fuzhou University, Fuzhou, 350116, China
  • [ 9 ] [Zheng, Y.]College of Chemistry, Fuzhou University, Fuzhou, 350116, China

Reprint 's Address:

  • [Zheng, Y.]College of Chemistry, Fuzhou UniversityChina

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Source :

Applied Catalysis B: Environmental

ISSN: 0926-3373

Year: 2020

Volume: 260

1 9 . 5 0 3

JCR@2020

2 0 . 3 0 0

JCR@2023

ESI HC Threshold:160

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 23

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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