Higher Alcohol Synthesis Over Rh Catalysts: Conditioning of Rh/N-CNTs by Co and Mn Entrapped in the Support - Details

author：

Xie, Z. (Xie, Z..) ^[1] | Frank, B. (Frank, B..) ^[2] | Huang, X. (Huang, X..) ^[3] | Schlögl, R. (Schlögl, R..) ^[4] | Trunschke, A. (Trunschke, A..) ^[5]

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Abstract：

Abstract:　Rh　nanoparticles　supported　on　commercial　non-purified　N-doped　CNTs　(NCNTs)　containing　residual　CNT　growth　catalyst　have　been　studied　in　hydrogenation　of　CO　to　higher　alcohols.　It　has　been　found　that　Co　and　Mn　residues　in　NCNTs　are　not　inert,　but　change　the　catalyst　under　reaction　conditions　and　efficiently　promote　the　catalyst　resulting　in　both　increasing　activity　and　selectivity　to　C2+　alcohols　with　time　on　stream.　Graphical　Abstract:　[Figure　not　available:　see　fulltext.]　©　2016,　The　Author(s).

Keyword：

Carbon nanotubes; CNT growth catalyst; Cobalt; Higher alcohol synthesis; Manganese; Nanoparticles; Nitrogen doping; Rhodium

Community：

[ 1 ] [Xie, Z.]Department of Inorganic Chemistry, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4-6, Berlin, 14195, Germany
[ 2 ] [Xie, Z.]College of Chemsitry, Fuzhou University, Qishan Campus, 2 Xueyuan Road, Fuzhou, 350116, China
[ 3 ] [Frank, B.]Department of Inorganic Chemistry, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4-6, Berlin, 14195, Germany
[ 4 ] [Frank, B.]BasCat - UniCat BASF JointLab, Technische Universität Berlin, Sekr. EW K 01, Hardenbergstr. 36, Berlin, 10623, Germany
[ 5 ] [Huang, X.]Department of Inorganic Chemistry, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4-6, Berlin, 14195, Germany
[ 6 ] [Schlögl, R.]Department of Inorganic Chemistry, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4-6, Berlin, 14195, Germany
[ 7 ] [Trunschke, A.]Department of Inorganic Chemistry, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4-6, Berlin, 14195, Germany

Reprint 's Address：

[Trunschke, A.]Department of Inorganic Chemistry, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4-6, Germany

Email：

trunschke@fhi-berlin.mpg.de

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Source ：

Catalysis Letters

ISSN： 1011-372X

Year： 2016

Issue： 12

Volume： 146

Page： 2417-2424

2 . 7 9 9

JCR@2016

2 . 3 0 0

JCR@2023

ESI HC Threshold：235

JCR Journal Grade：2

CAS Journal Grade：4

Cited Count：

WoS CC Cited Count：

SCOPUS Cited Count： 12

ESI Highly Cited Papers on the List： 0 Unfold All

WanFang Cited Count：

Chinese Cited Count：

30 Days PV： 2

Affiliated Colleges：

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