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author：

Fu, Y. (Fu, Y..) [1] | Sun, L. (Sun, L..) [2] | Yang, H. (Yang, H..) [3] | Xu, L. (Xu, L..) [4] | Zhang, F. (Zhang, F..) [5] | Zhu, W. (Zhu, W..) [6]

Indexed by：

Scopus

Abstract：

The　Ni-doped　NH2-MIL-125(Ti)　catalyst　was　developed　for　the　photocatalytic　aerobic　oxidation　of　aromatic　alcohols　upon　visible　light　irradiation.　The　results　show　that　different　aromatic　alcohols　can　be　effectively　transformed　to　their　corresponding　aldehydes　with　almost　absolute　selectivity　using　O2　as　the　oxidant　over　Ni-doped　NH2-MIL-125(Ti)　upon　visible　light　irradiation.　Compared　with　the　parent　catalyst　NH2-MIL-125(Ti),　Ni-doped　NH2-MIL-125(Ti)　exhibits　a　significantly　enhanced　photocatalytic　activity　for　the　selective　oxidation　of　aromatic　alcohols.　Preliminary　studies　indicate　that　the　doping　of　Ni　nanoparticles　into　NH2-MIL-125(Ti)　could　improve　the　visible-light　harvesting,　charge-separation,　and　electron-transport　of　the　resultant　catalyst,　leading　to　the　enhanced　photocatalytic　activity.　The　current　work　provides　some　guidance　in　the　development　of　MOF-based　photocatalysts　for　organic　syntheses.　©　2016　Elsevier　B.V.

Keyword：

Metal-organic frameworks; Molecular oxygen; Photocatalysis; Selective alcohol oxidation; Visible light

Community：

  • [ 1 ] [Fu, Y.]Key Laboratory of the Ministry of Education for Advanced Catalysis Materials, Institute of Physical Chemistry, Zhejiang Normal University, Jinhua, 321004, China
  • [ 2 ] [Fu, Y.]State Key Laboratory of Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou, 350002, China
  • [ 3 ] [Sun, L.]Key Laboratory of the Ministry of Education for Advanced Catalysis Materials, Institute of Physical Chemistry, Zhejiang Normal University, Jinhua, 321004, China
  • [ 4 ] [Yang, H.]Key Laboratory of the Ministry of Education for Advanced Catalysis Materials, Institute of Physical Chemistry, Zhejiang Normal University, Jinhua, 321004, China
  • [ 5 ] [Xu, L.]Key Laboratory of the Ministry of Education for Advanced Catalysis Materials, Institute of Physical Chemistry, Zhejiang Normal University, Jinhua, 321004, China
  • [ 6 ] [Zhang, F.]Key Laboratory of the Ministry of Education for Advanced Catalysis Materials, Institute of Physical Chemistry, Zhejiang Normal University, Jinhua, 321004, China
  • [ 7 ] [Zhu, W.]Key Laboratory of the Ministry of Education for Advanced Catalysis Materials, Institute of Physical Chemistry, Zhejiang Normal University, Jinhua, 321004, China

Reprint 's Address：

  • [Zhu, W.]Key Laboratory of the Ministry of Education for Advanced Catalysis Materials, Institute of Physical Chemistry, Zhejiang Normal UniversityChina

Email：


weidongzhu@zjnu.cn
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Source ：

Applied Catalysis B: Environmental

ISSN： 0926-3373

Year： 2016

Volume： 187

Page： 212-217

9 . 4 4 6

JCR@2016

2 0 . 3 0 0

JCR@2023

ESI HC Threshold：235

JCR Journal Grade：1

CAS Journal Grade：1

Cited Count：

WoS CC Cited Count：

SCOPUS Cited Count： 150

ESI Highly Cited Papers on the List： 0 Unfold All

WanFang Cited Count：

Chinese Cited Count：

30 Days PV： 3

Affiliated Colleges：

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