Introduction of a mediator for enhancing photocatalytic performance via post-synthetic metal exchange in metal-organic frameworks (MOFs) - Details

author：

Sun, D. (Sun, D..) ^[1] | Liu, W. (Liu, W..) ^[2] | Qiu, M. (Qiu, M..) ^[3] | Zhang, Y. (Zhang, Y..) ^[4] | Li, Z. (Li, Z..) ^[5]

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Abstract：

Ti-substituted　NH2-Uio-66(Zr/Ti)　prepared　by　using　a　post-synthetic　exchange　(PSE)　method　showed　enhanced　photocatalytic　performance　for　both　CO2　reduction　and　hydrogen　evolution　under　visible　light.　Density　functional　theory　(DFT)　calculations　and　electron　spin　resonance　(ESR)　results　reveal　that　the　introduced　Ti　substituent　acts　as　a　mediator　to　facilitate　electron　transfer,　which　results　in　enhanced　performance.　This　journal　is　©　The　Royal　Society　of　Chemistry.

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[ 1 ] [Sun, D.]Research Institute of Photocatalysis, State Key Laboratory of Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou, 350002, China
[ 2 ] [Liu, W.]Research Institute of Photocatalysis, State Key Laboratory of Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou, 350002, China
[ 3 ] [Qiu, M.]College of Chemistry, Fuzhou University, Fuzhou, 350002, China
[ 4 ] [Zhang, Y.]College of Chemistry, Fuzhou University, Fuzhou, 350002, China
[ 5 ] [Li, Z.]Research Institute of Photocatalysis, State Key Laboratory of Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou, 350002, China
[ 6 ] [Li, Z.]College of Chemistry, Fuzhou University, Fuzhou, 350002, China

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[Zhang, Y.]College of Chemistry, Fuzhou UniversityChina

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Source ：

Chemical Communications

ISSN： 1359-7345

Year： 2015

Issue： 11

Volume： 51

Page： 2056-2059

6 . 5 6 7

JCR@2015

4 . 3 0 0

JCR@2023

ESI HC Threshold：265

JCR Journal Grade：1

CAS Journal Grade：2

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WoS CC Cited Count：

SCOPUS Cited Count： 370

ESI Highly Cited Papers on the List： 0 Unfold All

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Chinese Cited Count：

30 Days PV： 3

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