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Abstract:
采用氧化-还原共沉淀法制备了Pr掺杂的Ru/CeO2-PrO2氨合成催化剂,并运用N2物理吸附、X射线粉末衍射、H2程序升温还原、CO化学吸附、N2程序升温脱附、场发射扫描电镜、高分辨透射电镜和X射线光电子能谱等技术对其进行了表征,考察了Pr添加量对催化剂表面结构和性能的影响.结果表明,Pr掺杂对Ru/CeO2催化剂的比表面积和Ru分散度都有所影响.当CeO2中Pr掺杂量为4%时,在425oC,10MPa,10000h–1的反应条件下,氨合成转化频率可达到12.13×10–2s–1,较Ru/CeO2催化剂提高了58%,这主要归结于复合材料电子传导性能的提高.
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催化学报
ISSN: 0253-9837
CN: 21-1601/O6
Year: 2012
Issue: 03
Volume: 33
Page: 536-542
1 . 3 0 4
JCR@2012
1 5 . 7 0 0
JCR@2023
JCR Journal Grade:2
CAS Journal Grade:4
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SCOPUS Cited Count:
ESI Highly Cited Papers on the List: 0 Unfold All
WanFang Cited Count:
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30 Days PV: 2
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