Isotopic O-18/O-16 substitution study on the direct partial oxidation of CH4 to dimethyl ether over a Pt/Y2O3 catalyst using NO/O-2 as an oxidant - Details

author：

Ghampson, I. Tyrone (Ghampson, I. Tyrone.) ^[1] | Lundin, Sean-Thomas B. (Lundin, Sean-Thomas B..) ^[2] | Shishido, Tetsuya (Shishido, Tetsuya.) ^[3] | Oyama, S. Ted (Oyama, S. Ted.) ^[4]

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EI SCIE

Abstract：

The　direct　partial　oxidation　of　CH4　to　dimethyl　ether　(DME)　was　achieved　with　a　Pt/Y2O3　catalyst　using　a　mixture　of　NO　and　O-2.　The　actual　gas　composition　contained　a　mixture　of　NO　and　NO2,　with　no　decomposition　or　net　consumption　of　these　species.　Use　of　O-18(2)　confirmed　the　transfer　of　labeled　oxygen　from　O-2　to　CH4,　indicating　the　NO/NO2　mixture　worked　as　a　single　oxygen　atom　shuttle.

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Community：

[ 1 ] [Oyama, S. Ted]Fuzhou Univ, Sch Chem Engn, Fuzhou 350116, Peoples R China
[ 2 ] [Ghampson, I. Tyrone]Tokyo Metropolitan Univ, Grad Sch Urban Environm Sci, Dept Appl Chem Environm, 1-1 Minami Osawa, Hachioji, Tokyo 1920397, Japan
[ 3 ] [Shishido, Tetsuya]Tokyo Metropolitan Univ, Grad Sch Urban Environm Sci, Dept Appl Chem Environm, 1-1 Minami Osawa, Hachioji, Tokyo 1920397, Japan
[ 4 ] [Ghampson, I. Tyrone]Univ Tokyo, Dept Chem Syst Engn, Bunkyo Ku, 7-3-1 Hongo, Tokyo 1138656, Japan
[ 5 ] [Lundin, Sean-Thomas B.]Univ Tokyo, Dept Chem Syst Engn, Bunkyo Ku, 7-3-1 Hongo, Tokyo 1138656, Japan
[ 6 ] [Oyama, S. Ted]Univ Tokyo, Dept Chem Syst Engn, Bunkyo Ku, 7-3-1 Hongo, Tokyo 1138656, Japan
[ 7 ] [Oyama, S. Ted]Virginia Tech, Dept Chem Engn, Blacksburg, VA 24061 USA

Reprint 's Address：

大山茂生
[Oyama, S. Ted]Fuzhou Univ, Sch Chem Engn, Fuzhou 350116, Peoples R China;;[Oyama, S. Ted]Univ Tokyo, Dept Chem Syst Engn, Bunkyo Ku, 7-3-1 Hongo, Tokyo 1138656, Japan;;[Oyama, S. Ted]Virginia Tech, Dept Chem Engn, Blacksburg, VA 24061 USA

Email：

oyama@vt.edu

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Isotopic18O/16O substitution study on the direct partial oxidation of CH4to dimethyl ether over a Pt/Y2O3catalyst using NO/O2as an oxidant
2021，Catalysis Science and Technology

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Source ：

CATALYSIS SCIENCE & TECHNOLOGY

ISSN： 2044-4753

Year： 2021

Issue： 8

Volume： 11

Page： 2708-2712

6 . 1 7 7

JCR@2021

4 . 4 0 0

JCR@2023

ESI Discipline： CHEMISTRY;

ESI HC Threshold：117

JCR Journal Grade：2

CAS Journal Grade：3

Cited Count：

WoS CC Cited Count： 0

SCOPUS Cited Count： 5

ESI Highly Cited Papers on the List： 0 Unfold All

WanFang Cited Count：

Chinese Cited Count：

30 Days PV： 0

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