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author：

Jia, Xiaoxia (Jia, Xiaoxia.) [1] | Zhao, Jiwu (Zhao, Jiwu.) [2] | Lv, Yujing (Lv, Yujing.) [3] | Fu, Xianliang (Fu, Xianliang.) [4] | Jian, Yajun (Jian, Yajun.) [5] | Zhang, Weiqiang (Zhang, Weiqiang.) [6] | Wang, Yanyan (Wang, Yanyan.) [7] | Sun, Huaming (Sun, Huaming.) [8] | Wang, Xuxu (Wang, Xuxu.) [9] | Long, Jinlin (Long, Jinlin.) [10] | Yang, Peng (Yang, Peng.) [11] | Gu, Quan (Gu, Quan.) [12] | Gao, Ziwei (Gao, Ziwei.) [13]

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EI

Abstract：

We　develop　a　new　PdCu/UTCN　hybrid　by　loading　low-crystalline　PdCu　NPs　on　large-area　ultrathin　2D　carbon　nitride　(UTCN)　nanosheets　that　exfoliated　from　bulk　g-C3N4　using　a　twice　thermal　exfoliation　and　repolymerization　method　for　photocatalytic　Suzuki　C-C　cross　coupling　reaction.　Due　to　the　advantages　of　2D　structure　of　the　UTCN　and　the　changes　in　electronic　structure　and　surface　structure　of　low-crystalline　PdCu　NPs,　PdCu/UTCN　shows　promoted　photocatalytic　activity　with　high　selectivity　for　Suzuki　coupling　reaction.　The　TOF　value　for　coupling　of　iodobenzene　with　phenylboronic　acid　is　418.2　h−1,　which　is　8　and　6.2　times　higher　than　that　of　previously　reported　Pd-g-C3N4　and　Pd　based　alloy　photocatalysts　under　the　same　reaction,　respectively.　Morevoer,　this　photocatalyst　shows　a　good　functional　group　tolerance　as　well　as　good　to　excellent　yield　and　selectivity　for　various　substrates.　This　study　reports　for　the　first　time　the　PdCu　alloy　supported　UTCN　photocatalytic　material　for　enhanced　Suzuki　reaction.　©　2021　Elsevier　B.V.

Keyword：

Binary alloys Carbon nitride Copper alloys Electronic structure Nanosheets Palladium alloys Photocatalytic activity Surface structure

Community：

  • [ 1 ] [Jia, Xiaoxia]Key Laboratory of Applied Surface and Colloid Chemistry, Ministry of Education, Xi'an Key Laboratory of Organometallic Material Chemistry, School of Chemistry and Chemical Engineering, Shaanxi Normal University, Xi'an; 710062, China
  • [ 2 ] [Zhao, Jiwu]State Key Laboratory of Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou; 350002, China
  • [ 3 ] [Lv, Yujing]Key Laboratory of Applied Surface and Colloid Chemistry, Ministry of Education, Xi'an Key Laboratory of Organometallic Material Chemistry, School of Chemistry and Chemical Engineering, Shaanxi Normal University, Xi'an; 710062, China
  • [ 4 ] [Fu, Xianliang]College of Chemistry and Material Science, Huaibei Normal University, Huaibei; Anhui; 235000, China
  • [ 5 ] [Jian, Yajun]Key Laboratory of Applied Surface and Colloid Chemistry, Ministry of Education, Xi'an Key Laboratory of Organometallic Material Chemistry, School of Chemistry and Chemical Engineering, Shaanxi Normal University, Xi'an; 710062, China
  • [ 6 ] [Zhang, Weiqiang]Key Laboratory of Applied Surface and Colloid Chemistry, Ministry of Education, Xi'an Key Laboratory of Organometallic Material Chemistry, School of Chemistry and Chemical Engineering, Shaanxi Normal University, Xi'an; 710062, China
  • [ 7 ] [Wang, Yanyan]Key Laboratory of Applied Surface and Colloid Chemistry, Ministry of Education, Xi'an Key Laboratory of Organometallic Material Chemistry, School of Chemistry and Chemical Engineering, Shaanxi Normal University, Xi'an; 710062, China
  • [ 8 ] [Sun, Huaming]Key Laboratory of Applied Surface and Colloid Chemistry, Ministry of Education, Xi'an Key Laboratory of Organometallic Material Chemistry, School of Chemistry and Chemical Engineering, Shaanxi Normal University, Xi'an; 710062, China
  • [ 9 ] [Wang, Xuxu]State Key Laboratory of Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou; 350002, China
  • [ 10 ] [Long, Jinlin]State Key Laboratory of Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou; 350002, China
  • [ 11 ] [Yang, Peng]Key Laboratory of Applied Surface and Colloid Chemistry, Ministry of Education, Xi'an Key Laboratory of Organometallic Material Chemistry, School of Chemistry and Chemical Engineering, Shaanxi Normal University, Xi'an; 710062, China
  • [ 12 ] [Gu, Quan]Key Laboratory of Applied Surface and Colloid Chemistry, Ministry of Education, Xi'an Key Laboratory of Organometallic Material Chemistry, School of Chemistry and Chemical Engineering, Shaanxi Normal University, Xi'an; 710062, China
  • [ 13 ] [Gao, Ziwei]Key Laboratory of Applied Surface and Colloid Chemistry, Ministry of Education, Xi'an Key Laboratory of Organometallic Material Chemistry, School of Chemistry and Chemical Engineering, Shaanxi Normal University, Xi'an; 710062, China

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Source ：

Applied Catalysis B: Environmental

ISSN： 0926-3373

Year： 2022

Volume： 300

2 2 . 1

JCR@2022

2 0 . 3 0 0

JCR@2023

ESI HC Threshold：74

JCR Journal Grade：1

CAS Journal Grade：1

Cited Count：

WoS CC Cited Count：

SCOPUS Cited Count： 34

ESI Highly Cited Papers on the List： 0 Unfold All

WanFang Cited Count：

Chinese Cited Count：

30 Days PV： 2

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