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author:

Zhang, Xuesong (Zhang, Xuesong.) [1] | Li, Yuguang (Li, Yuguang.) [2] | Li, Changxiang (Li, Changxiang.) [3] | Yang, Fan (Yang, Fan.) [4] | Jiang, Zhengming (Jiang, Zhengming.) [5] | Xue, Liyan (Xue, Liyan.) [6] | Shao, Zhiheng (Shao, Zhiheng.) [7] | Zhao, Zhigang (Zhao, Zhigang.) [8] | Xie, Meiying (Xie, Meiying.) [9] | Yu, Shuwen (Yu, Shuwen.) [10]

Indexed by:

EI

Abstract:

In this study, a new type of (La0.2Ce0.2Gd0.2Er0.2Tm0.2)2(WO4)3 single-phase high-entropy ceramic (HEC) powder was designed, prepared by solid-phase synthesis, and evenly mixed into an epoxy resin (EP) matrix to test the thermal neutron and γ-ray shielding performance. In terms of γ-ray shielding, (La0.2Ce0.2Gd0.2Er0.2Tm0.2)2(WO4)3 showed a higher lead equivalent value than EP at 65 keV, indicating a clear shielding effect in the feeble absorbing area of lead-based and bismuth-based materials; moreover, (La0.2Ce0.2Gd0.2Er0.2Tm0.2)2(WO4)3 showed good γ-ray shielding performance in both low-energy and medium-energy regions. In terms of thermal neutron shielding, the composite with the highest HEC content (EP/W3) had a nearly 100% shielding efficiency, while that of EP was approximately 50%, indicating that this material has favorable thermal neutron and γ-ray shielding performance. Moreover, the thermal conductivity of the resulting composite material was lower than 0.3 W·m−1·K−1, the tensile strength was higher than 10 MPa, and the density was lower than 1.5 g·cm−3. All these results suggest that (La0.2Ce0.2Gd0.2Er0.2Tm0.2)2(WO4)3 is a candidate radiation shielding material. © 2021 The Authors

Keyword:

Entropy Epoxy resins Gadolinium compounds Gamma rays Lanthanum compounds Neutrons Radiation shielding Rare earths Synthesis (chemical) Tensile strength Thermal conductivity

Community:

  • [ 1 ] [Zhang, Xuesong]Fujian Province Joint Innovation Key Laboratory of Fuel and Materials in Clean Nuclear Energy System, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 2 ] [Zhang, Xuesong]Ganjiang Innovation Academy, Chinese Academy of Sciences, Jiangxi Institute of Rare Earths, Chinese Academy of Sciences, Ganzhou; 341000, China
  • [ 3 ] [Zhang, Xuesong]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, and Fujian Provincial Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 4 ] [Zhang, Xuesong]Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials, Xiamen Institute of Rare Earth Materials, Haixi Institute, Chinese Academy of Sciences, Xiamen; 361021, China
  • [ 5 ] [Zhang, Xuesong]College of Chemical Engineering, Fuzhou University, Fuzhou; 350002, China
  • [ 6 ] [Li, Yuguang]Science and Technology on Reactor System Design Technology Laboratory, Nuclear Power Institute of China, Chengdu; 610213, China
  • [ 7 ] [Li, Changxiang]Science and Technology on Reactor System Design Technology Laboratory, Nuclear Power Institute of China, Chengdu; 610213, China
  • [ 8 ] [Yang, Fan]Fujian Province Joint Innovation Key Laboratory of Fuel and Materials in Clean Nuclear Energy System, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 9 ] [Yang, Fan]Ganjiang Innovation Academy, Chinese Academy of Sciences, Jiangxi Institute of Rare Earths, Chinese Academy of Sciences, Ganzhou; 341000, China
  • [ 10 ] [Yang, Fan]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, and Fujian Provincial Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 11 ] [Yang, Fan]Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials, Xiamen Institute of Rare Earth Materials, Haixi Institute, Chinese Academy of Sciences, Xiamen; 361021, China
  • [ 12 ] [Jiang, Zhengming]Fujian Province Joint Innovation Key Laboratory of Fuel and Materials in Clean Nuclear Energy System, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 13 ] [Jiang, Zhengming]Ganjiang Innovation Academy, Chinese Academy of Sciences, Jiangxi Institute of Rare Earths, Chinese Academy of Sciences, Ganzhou; 341000, China
  • [ 14 ] [Jiang, Zhengming]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, and Fujian Provincial Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 15 ] [Jiang, Zhengming]Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials, Xiamen Institute of Rare Earth Materials, Haixi Institute, Chinese Academy of Sciences, Xiamen; 361021, China
  • [ 16 ] [Xue, Liyan]Fujian Province Joint Innovation Key Laboratory of Fuel and Materials in Clean Nuclear Energy System, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 17 ] [Xue, Liyan]Ganjiang Innovation Academy, Chinese Academy of Sciences, Jiangxi Institute of Rare Earths, Chinese Academy of Sciences, Ganzhou; 341000, China
  • [ 18 ] [Xue, Liyan]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, and Fujian Provincial Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 19 ] [Xue, Liyan]Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials, Xiamen Institute of Rare Earth Materials, Haixi Institute, Chinese Academy of Sciences, Xiamen; 361021, China
  • [ 20 ] [Shao, Zhiheng]Fujian Province Joint Innovation Key Laboratory of Fuel and Materials in Clean Nuclear Energy System, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 21 ] [Shao, Zhiheng]Ganjiang Innovation Academy, Chinese Academy of Sciences, Jiangxi Institute of Rare Earths, Chinese Academy of Sciences, Ganzhou; 341000, China
  • [ 22 ] [Shao, Zhiheng]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, and Fujian Provincial Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 23 ] [Shao, Zhiheng]Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials, Xiamen Institute of Rare Earth Materials, Haixi Institute, Chinese Academy of Sciences, Xiamen; 361021, China
  • [ 24 ] [Zhao, Zhigang]Fujian Province Joint Innovation Key Laboratory of Fuel and Materials in Clean Nuclear Energy System, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 25 ] [Zhao, Zhigang]Ganjiang Innovation Academy, Chinese Academy of Sciences, Jiangxi Institute of Rare Earths, Chinese Academy of Sciences, Ganzhou; 341000, China
  • [ 26 ] [Zhao, Zhigang]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, and Fujian Provincial Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 27 ] [Zhao, Zhigang]Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials, Xiamen Institute of Rare Earth Materials, Haixi Institute, Chinese Academy of Sciences, Xiamen; 361021, China
  • [ 28 ] [Xie, Meiying]Fujian Province Joint Innovation Key Laboratory of Fuel and Materials in Clean Nuclear Energy System, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 29 ] [Xie, Meiying]Ganjiang Innovation Academy, Chinese Academy of Sciences, Jiangxi Institute of Rare Earths, Chinese Academy of Sciences, Ganzhou; 341000, China
  • [ 30 ] [Xie, Meiying]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, and Fujian Provincial Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 31 ] [Xie, Meiying]Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials, Xiamen Institute of Rare Earth Materials, Haixi Institute, Chinese Academy of Sciences, Xiamen; 361021, China
  • [ 32 ] [Yu, Shuwen]Fujian Province Joint Innovation Key Laboratory of Fuel and Materials in Clean Nuclear Energy System, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 33 ] [Yu, Shuwen]Ganjiang Innovation Academy, Chinese Academy of Sciences, Jiangxi Institute of Rare Earths, Chinese Academy of Sciences, Ganzhou; 341000, China
  • [ 34 ] [Yu, Shuwen]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, and Fujian Provincial Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350002, China
  • [ 35 ] [Yu, Shuwen]Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials, Xiamen Institute of Rare Earth Materials, Haixi Institute, Chinese Academy of Sciences, Xiamen; 361021, China

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Source :

Materials and Design

ISSN: 0264-1275

Year: 2021

Volume: 205

9 . 4 1 7

JCR@2021

7 . 6 0 0

JCR@2023

ESI HC Threshold:142

JCR Journal Grade:1

CAS Journal Grade:3

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 24

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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