Selective　removal　of　carbonyl　sulfide　(COS)　and　hydrogen　sulfide　(H2S)　is　the　key　step　for　natural　gas　desulfurization　due　to　thehighly　toxic　and　corrosive　features　of　these　gaseous　sulfides,　and　efficientand　stable　desulfurizers　are　urgently　needed　in　the　industry.　Herein,　wereport　a　class　of　nitrogen-functionalized,　hierarchically　lamellar　carbonframeworks　(N-HLCF-xs),　which　are　obtained　from　the　structuraltransformation　of　Zn　zeolitic　imidazolate　frameworks　via　controllablecarbonization.　The　N-HLCF-xs　possess　the　desirable　characteristics　oflarge　Brunauer-Emmett-Teller　surface　areas　(645-923　m2/g),　combinedprimary　three-dimensional　microporosity　and　secondary　two-dimensionallamellar　microstructure,　and　high　density　of　nitrogen　base　sites　withenhanced　pyridine　ratio　(17.52　wt　%,　59.91%).　The　anchored　nitrogenbase　sites　in　N-HLCF-xs　show　improved　accessibility,　which　boosts　theirinteraction　with　acidic　COS　and　H2S.　As　expected,　N-HLCF-xs　can　beemployed　as　multifunctional　and　efficient　desulfurizers　for　selective　removal　of　COS　and　H2S　from　natural　gas.　COS　wasfirsttransformed　into　H2S　via　catalytic　hydrolysis,　and　the　produced　H2S　was　then　captured　and　separated　and　catalyzed　oxidation　intoelemental　sulfur.　The　above　continuous　processes　can　be　achieved　with　solo　N-HLCF-xs,　giving　extremely　high　efficiencies　andreusability.　Their　integrated　desulfurization　performance　was　better　than　many　desulfurizers　used　in　the　area,　such　as　activatedcarbon,beta　zeolite,　MIL-101(Fe),　K2CO3/gamma-Al2O3,　and　FeOx/TiO2