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author:

Zhou, Pengfei (Zhou, Pengfei.) [1] | Niu, Pengda (Niu, Pengda.) [2] | Liu, Jishan (Liu, Jishan.) [3] | Zhang, Nian (Zhang, Nian.) [4] | Bai, Haoyun (Bai, Haoyun.) [5] | Chen, Mingpeng (Chen, Mingpeng.) [6] | Feng, Jinxian (Feng, Jinxian.) [7] | Liu, Di (Liu, Di.) [8] | Wang, Litong (Wang, Litong.) [9] | Chen, Shi (Chen, Shi.) [10] | Kwok, Chi Tat (Kwok, Chi Tat.) [11] | Tang, Yuxin (Tang, Yuxin.) [12] | Li, Ruidi (Li, Ruidi.) [13] | Wang, Shuangpeng (Wang, Shuangpeng.) [14] | Pan, Hui (Pan, Hui.) [15]

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EI

Abstract:

Electrolysis of water, especially alkaline water electrolysis (AWE), is the most promising technology to produce hydrogen in industry. However, only 4% of the total hydrogen is produced in this way because the electrode materials are expensive, inefficient, or unstable. Here, it is reported that the large-scale 3D printed martensitic steel (AerMet100) can be the bifunctional electrode for AWE with high catalytic performance, which may dramatically increase the green-hydrogen percentage in the market and provide strategic planning for energy management. It is found that the martensitic steel by fast anodization (3 min) can realize ultra-high hydrogen and oxygen evolution reactions (HER and OER), and excellent stability at high current densities. Particularly, this electrocatalyst shows a low overpotential of 3.18 V and long-term stability over 140 h at 570 mA cm−2 in overall water splitting. Additionally, the treated large-scale steel can work well under a very high current up to 20 A. This study demonstrates that martensitic steel can be commercialized as a highly efficient catalyst for industrial hydrogen production in AWE, which should provide solutions to the energy crisis and environmental pollution. © 2022 Wiley-VCH GmbH.

Keyword:

3D printers Electrocatalysis Electrocatalysts Electrodes Electrolysis Energy policy Hydrogen production Martensitic stainless steel

Community:

  • [ 1 ] [Zhou, Pengfei]Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, 999078, China
  • [ 2 ] [Niu, Pengda]Science and Technology on High Strength Structural Materials Laboratory, State Key Laboratory of Powder Metallurgy, Central South University, 932 Lushan S Rd, Yuelu District, Changsha; 410083, China
  • [ 3 ] [Liu, Jishan]State Key Laboratory of Functional Materials for Informatics, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences, Shanghai; 200050, China
  • [ 4 ] [Zhang, Nian]State Key Laboratory of Functional Materials for Informatics, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences, Shanghai; 200050, China
  • [ 5 ] [Bai, Haoyun]Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, 999078, China
  • [ 6 ] [Chen, Mingpeng]Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, 999078, China
  • [ 7 ] [Feng, Jinxian]Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, 999078, China
  • [ 8 ] [Liu, Di]Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, 999078, China
  • [ 9 ] [Wang, Litong]Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, 999078, China
  • [ 10 ] [Chen, Shi]Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, 999078, China
  • [ 11 ] [Kwok, Chi Tat]Department of Electromechanical Engineering, Faculty of Science and Technology, University of Macau, Avenida da Universidade, Taipa, 999078, China
  • [ 12 ] [Tang, Yuxin]College of Chemical Engineering, Fuzhou University, Xueyuan Rd, Gulou District, Fuzhou; 350116, China
  • [ 13 ] [Li, Ruidi]Science and Technology on High Strength Structural Materials Laboratory, State Key Laboratory of Powder Metallurgy, Central South University, 932 Lushan S Rd, Yuelu District, Changsha; 410083, China
  • [ 14 ] [Wang, Shuangpeng]Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, 999078, China
  • [ 15 ] [Pan, Hui]Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, 999078, China
  • [ 16 ] [Pan, Hui]Department of Physics and Chemistry, Faculty of Science and Technology, University of Macau, Avenida da Universidade, Taipa, 999078, China

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Source :

Advanced Functional Materials

ISSN: 1616-301X

Year: 2022

Issue: 26

Volume: 32

1 9 . 0

JCR@2022

1 8 . 5 0 0

JCR@2023

ESI HC Threshold:91

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 52

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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