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author：

Huang, J. (Huang, J..) [1] | Sementa, L. (Sementa, L..) [2] | Liu, Z. (Liu, Z..) [3] | Barcaro, G. (Barcaro, G..) [4] | Feng, M. (Feng, M..) [5] | Liu, E. (Liu, E..) [6] | Jiao, L. (Jiao, L..) [7] | Xu, M. (Xu, M..) [8] | Leshchev, D. (Leshchev, D..) [9] | Lee, S.-J. (Lee, S.-J..) [10] | Li, M. (Li, M..) [11] | Wan, C. (Wan, C..) [12] | Zhu, E. (Zhu, E..) [13] | Liu, Y. (Liu, Y..) [14] | Peng, B. (Peng, B..) [15] | Duan, X. (Duan, X..) [16] | Goddard, W.A. (Goddard, W.A..) [17] | III (III.) [18] | Fortunelli, A. (Fortunelli, A..) [19] | Jia, Q. (Jia, Q..) [20] | Huang, Y. (Huang, Y..) [21]

Indexed by：

Scopus

Abstract：

A　critical　technological　roadblock　to　the　widespread　adoption　of　proton-exchange　membrane　fuel　cells　is　the　development　of　highly　active　and　durable　platinum-based　catalysts　for　accelerating　the　sluggish　oxygen　reduction　reaction,　which　has　largely　relied　on　anecdotal　discoveries　so　far.　While　the　oxygen　binding　energy　∆EO　has　been　frequently　used　as　a　theoretical　descriptor　for　predicting　the　activity,　there　is　no　known　descriptor　for　predicting　durability.　Here　we　developed　a　binary　experimental　descriptor　that　captures　both　the　strain　and　Pt　transition　metal　coupling　contributions　through　X-ray　absorption　spectroscopy　and　directly　correlated　the　binary　experimental　descriptor　with　the　calculated　∆EO　of　the　catalyst　surface.　This　leads　to　an　experimentally　validated　Sabatier　plot　to　predict　both　the　catalytic　activity　and　stability　for　a　wide　range　of　Pt-alloy　oxygen　reduction　reaction　catalysts.　Based　on　the　binary　experimental　descriptor,　we　further　designed　an　oxygen　reduction　reaction　catalyst　wherein　high　activity　and　stability　are　simultaneously　achieved.　[Figure　not　available:　see　fulltext.]　©　2022,　The　Author(s),　under　exclusive　licence　to　Springer　Nature　Limited.

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  • [ 1 ] [Huang, J.]Department of Materials Science and Engineering, University of California, Los Angeles, CA, United States
  • [ 2 ] [Sementa, L.]CNR-ICCOM & IPCF, Consiglio Nazionale delle Ricerche, Pisa, Italy
  • [ 3 ] [Liu, Z.]Department of Materials Science and Engineering, University of California, Los Angeles, CA, United States
  • [ 4 ] [Barcaro, G.]CNR-ICCOM & IPCF, Consiglio Nazionale delle Ricerche, Pisa, Italy
  • [ 5 ] [Feng, M.]Department of Materials Science and Engineering, University of California, Los Angeles, CA, United States
  • [ 6 ] [Feng, M.]College of Materials Science and Engineering, Fuzhou University, Fuzhou, China
  • [ 7 ] [Liu, E.]Department of Chemistry and Chemical Biology, Northeastern University, Boston, MA, United States
  • [ 8 ] [Jiao, L.]Department of Chemistry and Chemical Biology, Northeastern University, Boston, MA, United States
  • [ 9 ] [Xu, M.]Irvine Materials Research Institute, University of California, Irvine, CA, United States
  • [ 10 ] [Xu, M.]Department of Materials Science, University of California, Irvine, CA, United States
  • [ 11 ] [Leshchev, D.]National Synchrotron Light Source II, Brookhaven National Laboratory, Upton, NY, United States
  • [ 12 ] [Lee, S.-J.]Department of Materials Science and Engineering, University of California, Los Angeles, CA, United States
  • [ 13 ] [Li, M.]Department of Chemistry and Biochemistry, University of California, Los Angeles, CA, United States
  • [ 14 ] [Wan, C.]Department of Chemistry and Biochemistry, University of California, Los Angeles, CA, United States
  • [ 15 ] [Zhu, E.]Department of Materials Science and Engineering, University of California, Los Angeles, CA, United States
  • [ 16 ] [Liu, Y.]Department of Materials Science and Engineering, University of California, Los Angeles, CA, United States
  • [ 17 ] [Peng, B.]Department of Chemistry and Biochemistry, University of California, Los Angeles, CA, United States
  • [ 18 ] [Duan, X.]Department of Chemistry and Biochemistry, University of California, Los Angeles, CA, United States
  • [ 19 ] [Duan, X.]California NanoSystems Institute, University of California, Los Angeles, CA, United States
  • [ 20 ] [Goddard, W.A.]Materials and Process Simulation Center, California Institute of Technology, Pasadena, CA, United States
  • [ 21 ] [Fortunelli, A.]CNR-ICCOM & IPCF, Consiglio Nazionale delle Ricerche, Pisa, Italy
  • [ 22 ] [Jia, Q.]Department of Chemistry and Chemical Biology, Northeastern University, Boston, MA, United States
  • [ 23 ] [Huang, Y.]Department of Materials Science and Engineering, University of California, Los Angeles, CA, United States
  • [ 24 ] [Huang, Y.]California NanoSystems Institute, University of California, Los Angeles, CA, United States

Reprint 's Address：

  • [Huang, Y.]Department of Materials Science and Engineering, United States; ; CNR-ICCOM & IPCF, Italy; 电子邮件: alessandro.fortunelli@cnr.it Jia, Q.; Department of Chemistry and Chemical Biology, United States; 电子邮件: qjia@iit.edu Goddard, W.A.; Materials and Process Simulation Center, United States; 电子邮件: wag@wag.caltech.edu

Email：


yhuang@seas.ucla.edu Fortunelli, A.
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Source ：

Nature Catalysis

ISSN： 2520-1158

Year： 2022

Issue： 6

Volume： 5

Page： 513-523

3 7 . 8

JCR@2022

4 2 . 9 0 0

JCR@2023

ESI HC Threshold：74

JCR Journal Grade：1

CAS Journal Grade：1

Cited Count：

WoS CC Cited Count：

SCOPUS Cited Count：

ESI Highly Cited Papers on the List： 0 Unfold All

WanFang Cited Count：

Chinese Cited Count：

30 Days PV： 1

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