Heterostructured(HS)material　with　extraordinary　mechanical　properties　has　been　regarded　as　one　of　the　most　promising　structural　materials.Here,we　reported　a　new　strategy　for　preparing　heterostructured　pure　titanium　laminates　that　possess　a　good　combination　of　strength　and　ductility　by　combining　gradi-ent　structure(GS)and　heterogeneous　lamella　structure(HLS).The　deformation　characteristic　versus　mi-crostructure　evolution　of　GS/HLS　titanium　laminates,namely　the　strain　partitions　between　different-sized　grains(480-25　μm)was　visualized　using　a　scanning　electron　microscope(SEM)equipped　with　electron　backscattered　diffraction(EBSD)mode　combined　with　the　digital　image　correlation(SEM-DIC)with　an　ultrahigh　spatial　resolution　for　the　first　time.As　a　result,the　hetero-deformation　of　unique　GS/HLS　struc-ture　by　the　characteristic　of　strain　partitions　could　be　accurately　captured.While　the　hetero-deformation　could　result　in　the　hetero-deformation　induced(HDI)stress　strengthening　and　HDI　hardening,which　were　regarded　as　the　key　reason　that　the　resulting　GS/HLS　Ti　laminates　showed　a　superior　combina-tion　of　strength　and　ductility.This　could　promote　a　more　in-depth　understanding　of　the　strengthening-toughening　mechanism　of　heterostructured　material.