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Integrating high ionic conductivity and robust mechanical properties into one hydrogel remains challenging to date. In this paper, poly(vinyl alcohol)/carboxymethyl chitosan/tannic acid/NaCl/glycerol (PCTNG) organohydrogel was prepared by introducing tannic acid (TA), NaCl and glycerol (Gly) into poly(vinyl alcohol)/carboxymethyl chitosan (PVA/CMCS) simultaneously. Owing to the multiple hydrogen bonding complexations, the salting-out effect and metal coordination, the PCTNG organohydrogel showed an attractive overall performance with high tensile strength (2.02 MPa), large elongation at break (570.82%), superb ionic conductivity (3.05 S/m), excellent thermoplasticity and thermally assisted self-healing ability. Moreover, the introduction of Gly made PCTNG organohydrogel had high anti-freezing and anti-dehydration properties. The introduction of TA and NaCl endowed PCTNG organohydrogel with anti-bacterial properties. A flexible strain sensor was made based on this organoydrogel and this strain sensor could detect various human activities. This study provided a simple and promising strategy for manufacturing ionic conductive organohydrogel for flexible wearable devices. Graphical abstract: [Figure not available: see fulltext.] © 2022, The Author(s), under exclusive licence to Springer Nature B.V.
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Cellulose
ISSN: 0969-0239
Year: 2022
Issue: 17
Volume: 29
Page: 9323-9339
5 . 7
JCR@2022
4 . 9 0 0
JCR@2023
ESI HC Threshold:91
JCR Journal Grade:1
CAS Journal Grade:1
Cited Count:
SCOPUS Cited Count: 15
ESI Highly Cited Papers on the List: 0 Unfold All
WanFang Cited Count:
Chinese Cited Count:
30 Days PV: 2
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