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author:

Zhang, L. (Zhang, L..) [1] | Hu, O. (Hu, O..) [2] | Zhang, J. (Zhang, J..) [3] | Hou, L. (Hou, L..) [4] | Ye, D. (Ye, D..) [5] | Jiang, X. (Jiang, X..) [6] | Xiao, G. (Xiao, G..) [7]

Indexed by:

Scopus

Abstract:

Integrating high ionic conductivity and robust mechanical properties into one hydrogel remains challenging to date. In this paper, poly(vinyl alcohol)/carboxymethyl chitosan/tannic acid/NaCl/glycerol (PCTNG) organohydrogel was prepared by introducing tannic acid (TA), NaCl and glycerol (Gly) into poly(vinyl alcohol)/carboxymethyl chitosan (PVA/CMCS) simultaneously. Owing to the multiple hydrogen bonding complexations, the salting-out effect and metal coordination, the PCTNG organohydrogel showed an attractive overall performance with high tensile strength (2.02 MPa), large elongation at break (570.82%), superb ionic conductivity (3.05 S/m), excellent thermoplasticity and thermally assisted self-healing ability. Moreover, the introduction of Gly made PCTNG organohydrogel had high anti-freezing and anti-dehydration properties. The introduction of TA and NaCl endowed PCTNG organohydrogel with anti-bacterial properties. A flexible strain sensor was made based on this organoydrogel and this strain sensor could detect various human activities. This study provided a simple and promising strategy for manufacturing ionic conductive organohydrogel for flexible wearable devices. Graphical abstract: [Figure not available: see fulltext.] © 2022, The Author(s), under exclusive licence to Springer Nature B.V.

Keyword:

Anti-dehydration Ionic conductivity Salting-out effect Strain sensor Thermoplasticity

Community:

  • [ 1 ] [Zhang, L.]School of Chemical Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 2 ] [Hu, O.]School of Chemical Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 3 ] [Zhang, J.]School of Chemical Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 4 ] [Hou, L.]School of Chemical Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 5 ] [Ye, D.]State Key Laboratory of New Textile Materials and Advanced Processing Technologies, Wuhan Textile University, No. 1 Yangguang Avenue, Jiangxia District, Hubei, Wuhan, 430200, China
  • [ 6 ] [Jiang, X.]School of Chemical Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 7 ] [Jiang, X.]Qingyuan Innovation Laboratory, Quanzhou, 362114, China
  • [ 8 ] [Xiao, G.]College of Environment and Safety Engineering, Fuzhou University, Fuzhou, 350108, China

Reprint 's Address:

  • [Jiang, X.]School of Chemical Engineering, China;;[Ye, D.]State Key Laboratory of New Textile Materials and Advanced Processing Technologies, No. 1 Yangguang Avenue, Jiangxia District, Hubei, China;;[Xiao, G.]College of Environment and Safety Engineering, China

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Source :

Cellulose

ISSN: 0969-0239

Year: 2022

Issue: 17

Volume: 29

Page: 9323-9339

5 . 7

JCR@2022

4 . 9 0 0

JCR@2023

ESI HC Threshold:91

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 18

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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