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author：

Zhao, S. (Zhao, S..) [1] | Zhang, Y. (Zhang, Y..) [2] | Li, J. (Li, J..) [3] | Qi, L. (Qi, L..) [4] | Tang, Y. (Tang, Y..) [5] | Zhu, J. (Zhu, J..) [6] | Zhi, J. (Zhi, J..) [7] | Huang, F. (Huang, F..) [8]

Indexed by：

Scopus

Abstract：

Although　zinc-based　batteries　are　promising　candidates　for　eco-friendly　and　cost-effective　energy　storage　devices,　their　performance　is　severely　retarded　by　dendrite　formation.　As　the　simplest　zinc　compounds,　zinc　chalcogenides,　and　halides　are　individually　applied　as　a　Zn　protection　layer　due　to　high　zinc　ion　conductivity.　However,　the　mixed-anion　compounds　are　not　studied,　which　constrains　the　Zn2+　diffusion　in　single-anion　lattices　to　their　own　limits.　A　heteroanionic　zinc　ion　conductor　(ZnyO1−xFx)　coating　layer　is　designed　by　in　situ　growth　method　with　tunable　F　content　and　thickness.　Strengthened　by　F　aliovalent　doping,　the　Zn2+　conductivity　is　enhanced　within　the　wurtzite　motif　for　rapid　lattice　Zn　migration.　ZnyO1−xFx　also　affords　zincophilic　sites　for　oriented　superficial　Zn　plating　to　suppress　dendrite　growth.　Therefore,　ZnyO1−xFx-coated　anode　exhibits　a　low　overpotential　of　20.4 mV　for　1000 h　cycle　life　at　a　plating　capacity　of　1.0 mA h cm−2　during　symmetrical　cell　test.　The　MnO2//Zn　full　battery　further　proves　high　stability　of　169.7　mA h g−1　for　1000　cycles.　This　work　may　enlighten　the　mixed-anion　tuning　for　high-performance　Zn-based　energy　storage　devices.　©　2023　Wiley-VCH　GmbH.

Keyword：

anodization mixed anion compounds zinc anode protection zinc ion conductors

Community：

  • [ 1 ] [Zhao, S.]Beijing National Laboratory for Molecular Sciences and State Key Laboratory of Rare Earth Materials Chemistry and Applications, College of Chemistry and Molecular Engineering, Peking University, Beijing, 100871, China
  • [ 2 ] [Zhang, Y.]Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University, Beijing, 100871, China
  • [ 3 ] [Li, J.]College of Chemical Engineering, Fuzhou University, Fuzhou, 350116, China
  • [ 4 ] [Li, J.]Laboratory of Theoretical and Computational Nanoscience, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Chinese Academy of Sciences, Beijing, 100871, China
  • [ 5 ] [Qi, L.]Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering, Peking University, Beijing, 100871, China
  • [ 6 ] [Tang, Y.]College of Chemical Engineering, Fuzhou University, Fuzhou, 350116, China
  • [ 7 ] [Zhu, J.]Laboratory of Theoretical and Computational Nanoscience, CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Chinese Academy of Sciences, Beijing, 100871, China
  • [ 8 ] [Zhi, J.]State Key Laboratory of High-Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai, 200050, China
  • [ 9 ] [Huang, F.]Beijing National Laboratory for Molecular Sciences and State Key Laboratory of Rare Earth Materials Chemistry and Applications, College of Chemistry and Molecular Engineering, Peking University, Beijing, 100871, China
  • [ 10 ] [Huang, F.]State Key Laboratory of High-Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai, 200050, China

Reprint 's Address：

  • [Huang, F.]Beijing National Laboratory for Molecular Sciences and State Key Laboratory of Rare Earth Materials Chemistry and Applications, China;;[Zhi, J.]State Key Laboratory of High-Performance Ceramics and Superfine Microstructure, China

Email：


huangfq@mail.sic.ac.cn |
jzhi@mail.sic.ac.cn
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Source ：

Advanced Materials

ISSN： 0935-9648

Year： 2023

Issue： 18

Volume： 35

2 7 . 4

JCR@2023

2 7 . 4 0 0

JCR@2023

ESI HC Threshold：49

JCR Journal Grade：1

CAS Journal Grade：1

Cited Count：

WoS CC Cited Count：

SCOPUS Cited Count： 89

ESI Highly Cited Papers on the List： 0 Unfold All

WanFang Cited Count：

Chinese Cited Count：

30 Days PV： 5

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