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author:

He, Xuejie (He, Xuejie.) [1] | Shi, Shuohui (Shi, Shuohui.) [2] | Huang, Wei (Huang, Wei.) [3] | Fan, Xing (Fan, Xing.) [4] | Zhou, Jian (Zhou, Jian.) [5] | Chen, Yihong (Chen, Yihong.) [6] | Wang, Yingmu (Wang, Yingmu.) [7] (Scholars:王颖慕)

Indexed by:

EI Scopus SCIE

Abstract:

A novel electrolysis-integrated anammox (Ele-anammox) process was developed for intensified nitrogen removal and concomitant phosphorus recovery from nutrient-rich wastewater. By conducting a parallel experiment, average removal efficiencies of total nitrogen (TN) and total phosphorus (TP) in Ele-anammox reactor reached 90.69% and 95.02% respectively, showing increases of 7.76% and 79.08%, as compared to the traditional anammox process. Anammox reaction and synergetic denitrification were mainly responsible for the reinforced N-removal. Successions of microbial communities revealed that Candidatus Kuenenia declined markedly while Candidatus Brocadia was enriched in Ele-anammox system, suggesting that electrical environment provided Candidatus Brocadia with a competitive advantage over other anammox bacteria. Based on the proposed current control strategy (the applied current was calculated to match the influent P loading), precise release of soluble Fe2+ could be achieved by anodic oxidation. Various elemental analysis methods, including the standards, measurements and testing (SMT) protocol, energy dispersive X-ray spectroscopy (eSEM-EDX), X-ray fluorescence spectrometry (XRF) and inductively coupled plasma emission spectroscopy (ICP-OES), jointly indicated that the solid phase of Ele-anammox was primarily Fe-P precipitation, which showed a similar Fe:P ratio with vivianite (Fe-3(PO4)(2)center dot 8H(2)O, 1.5). X-ray diffraction (XRD) analysis further validated the in-situ crystallization of vivianite, and semi-quantification implied a vivianite content of 85%. Mossbauer spectroscopy showed at least 51.48% similar to 59.11% of iron was bound in vivianite, while impurity occupation and potential oxidization may impair the purity of P-recovery products, which should be concerned in future practice.

Keyword:

Anammox Electrolysis Nutrients removal Phosphorus recovery Vivianite

Community:

  • [ 1 ] [He, Xuejie]Chongqing Univ, Key Lab Three Gorges Reservoir Reg Ecoenvironm, Minist Educ, Chongqing 400045, Peoples R China
  • [ 2 ] [Shi, Shuohui]Chongqing Univ, Key Lab Three Gorges Reservoir Reg Ecoenvironm, Minist Educ, Chongqing 400045, Peoples R China
  • [ 3 ] [Huang, Wei]Chongqing Univ, Key Lab Three Gorges Reservoir Reg Ecoenvironm, Minist Educ, Chongqing 400045, Peoples R China
  • [ 4 ] [Fan, Xing]Chongqing Univ, Key Lab Three Gorges Reservoir Reg Ecoenvironm, Minist Educ, Chongqing 400045, Peoples R China
  • [ 5 ] [Zhou, Jian]Chongqing Univ, Key Lab Three Gorges Reservoir Reg Ecoenvironm, Minist Educ, Chongqing 400045, Peoples R China
  • [ 6 ] [Chen, Yihong]Chongqing Univ, Key Lab Three Gorges Reservoir Reg Ecoenvironm, Minist Educ, Chongqing 400045, Peoples R China
  • [ 7 ] [Wang, Yingmu]Fuzhou Univ, Coll Civil Engn, Fuzhou 350116, Fujian, Peoples R China

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Source :

CHEMICAL ENGINEERING JOURNAL

ISSN: 1385-8947

Year: 2023

Volume: 466

1 3 . 4

JCR@2023

1 3 . 4 0 0

JCR@2023

ESI Discipline: ENGINEERING;

ESI HC Threshold:35

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 5

SCOPUS Cited Count: 6

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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