2D MXenes polar catalysts for multi-renewable energy harvesting applications - Details

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The　synchronous　harvesting　and　conversion　of　multiple　renewable　energy　sources　for　chemical　fuel　production　and　environmental　remediation　in　a　single　system　is　a　holy　grail　in　sustainable　energy　technologies.　However,　it　is　challenging　to　develop　advanced　energy　harvesters　that　satisfy　different　working　mechanisms.　Here,　we　theoretically　and　experimentally　disclose　the　use　of　MXene　materials　as　versatile　catalysts　for　multi-energy　utilization.　Ti3C2TX　MXene　shows　remarkable　catalytic　performance　for　organic　pollutant　decomposition　and　H2　production.　It　outperforms　most　reported　catalysts　under　the　stimulation　of　light,　thermal,　and　mechanical　energy.　Moreover,　the　synergistic　effects　of　piezo-thermal　and　piezo-photothermal　catalysis　further　improve　the　performance　when　using　Ti3C2TX.　A　mechanistic　study　reveals　that　hydroxyl　and　superoxide　radicals　are　produced　on　the　Ti3C2TX　under　diverse　energy　stimulation.　Furthermore,　similar　multi-functionality　is　realized　in　Ti2CTX,　V2CTX,　and　Nb2CTX　MXene　materials.　This　work　is　anticipated　to　open　a　new　avenue　for　multisource　renewable　energy　harvesting　using　MXene　materials.　©　2023.　The　Author(s).

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[ 1 ] [Pan X.]College of Chemical Engneering and Materials, Quanzhou Normal University, Quanzhou, 362000, China
[ 2 ] [Yang X.]College of Environmental and Resource Sciences, College of Carbon Neutral Modern Industry, Fujian Key Laboratory of Pollution Control & Resource Reuse, Fujian Normal University, Fuzhou, 350007, China
[ 3 ] [Yu M.]College of Chemical Engneering and Materials, Quanzhou Normal University, Quanzhou, 362000, China
[ 4 ] [Yu M.]National Engineering Research Center of Chemical Fertilizer Catalyst Fuzhou University, Fuzhou, 350002, China
[ 5 ] [Lu X.]College of Chemical Engneering and Materials, Quanzhou Normal University, Quanzhou, 362000, China
[ 6 ] [Lu X.]College of Environmental and Resource Sciences, College of Carbon Neutral Modern Industry, Fujian Key Laboratory of Pollution Control & Resource Reuse, Fujian Normal University, Fuzhou, 350007, China
[ 7 ] [Kang H.]College of Environmental and Resource Sciences, College of Carbon Neutral Modern Industry, Fujian Key Laboratory of Pollution Control & Resource Reuse, Fujian Normal University, Fuzhou, 350007, China
[ 8 ] [Yang M.-Q.]College of Environmental and Resource Sciences, College of Carbon Neutral Modern Industry, Fujian Key Laboratory of Pollution Control & Resource Reuse, Fujian Normal University, Fuzhou, 350007, China
[ 9 ] [Qian Q.]College of Environmental and Resource Sciences, College of Carbon Neutral Modern Industry, Fujian Key Laboratory of Pollution Control & Resource Reuse, Fujian Normal University, Fuzhou, 350007, China
[ 10 ] [Zhao X.]College of Chemical Engneering and Materials, Quanzhou Normal University, Quanzhou, 362000, China
[ 11 ] [Liang S.]National Engineering Research Center of Chemical Fertilizer Catalyst Fuzhou University, Fuzhou, 350002, China
[ 12 ] [Bian Z.]Education Ministry Key and International Joint Lab of Resource Chemistry and Shanghai Key Lab of Rare Earth Functional Materials, Shanghai Normal University, 200234, Shanghai, China

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Nature communications

ISSN： 2041-1723

Year： 2023

Issue： 1

Volume： 14

Page： 4183-

1 4 . 7

JCR@2023

1 4 . 7 0 0

JCR@2023

ESI HC Threshold：42

JCR Journal Grade：1

CAS Journal Grade：1

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SCOPUS Cited Count： 26

ESI Highly Cited Papers on the List： 0 Unfold All

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30 Days PV： 0

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