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author:

Wu, Q. (Wu, Q..) [1] | Xu, Y. (Xu, Y..) [2] | Han, S. (Han, S..) [3] | Zhu, J. (Zhu, J..) [4] | Chen, A. (Chen, A..) [5] | Zhang, J. (Zhang, J..) [6] | Chen, Y. (Chen, Y..) [7] | Yang, X. (Yang, X..) [8] | Huang, J. (Huang, J..) [9] | Guan, L. (Guan, L..) [10]

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Abstract:

Conductive elastomers with both softness and conductivity are widely used in the field of flexible electronics. Nonetheless, conductive elastomers typically exhibit prominent problems such as solvent volatilization and leakage, and poor mechanical and conductive properties, which limit their applications in electronic skin (e-skin). In this work, a liquid-free conductive ionogel (LFCIg) with excellent performance was fabricated by utilizing the innovative double network design approach based on a deep eutectic solvent (DES). The double-network LFCIg is cross-linked by dynamic non-covalent bonds, which exhibit excellent mechanical properties (2100% strain while sustaining a fracture strength of 1.23 MPa) and >90% self-healing efficiency, and a superb electrical conductivity of 23.3 mS m−1 and 3D printability. Moreover, the conductive elastomer based on LFCIg has been developed into a stretchable strain sensor that achieves accurate response recognition, classification, and identification of different robot gestures. More impressively, an e-skin with tactile sensing functions is produced by in situ 3D printing of sensor arrays on flexible electrodes to detect light weight objects and recognize the resulting spatial pressure variations. Collectively, the results demonstrate that the designed LFCIg has unparalleled advantages and presents wide application potential in flexible robotics, e-skin and physiological signal monitoring. © 2023 The Royal Society of Chemistry.

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  • [ 1 ] [Wu Q.]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, Fujian Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350108, China
  • [ 2 ] [Wu Q.]School of Mechanical Engineering and Automation, Fuzhou University, Fuzhou, 350108, China
  • [ 3 ] [Xu Y.]Department of Oncology, The First Affiliated Hospital of Anhui Medical University, Hefei, 230000, China
  • [ 4 ] [Han S.]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, Fujian Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350108, China
  • [ 5 ] [Han S.]School of Mechanical Engineering and Automation, Fuzhou University, Fuzhou, 350108, China
  • [ 6 ] [Zhu J.]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, Fujian Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350108, China
  • [ 7 ] [Chen A.]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, Fujian Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350108, China
  • [ 8 ] [Zhang J.]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, Fujian Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350108, China
  • [ 9 ] [Chen Y.]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, Fujian Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350108, China
  • [ 10 ] [Yang X.]School of Mechanical Engineering and Automation, Fuzhou University, Fuzhou, 350108, China
  • [ 11 ] [Huang J.]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, Fujian Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350108, China
  • [ 12 ] [Huang J.]School of Mechanical Engineering and Automation, Fuzhou University, Fuzhou, 350108, China
  • [ 13 ] [Guan L.]CAS Key Laboratory of Design and Assembly of Functional Nanostructures, Fujian Key Laboratory of Nanomaterials, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350108, China
  • [ 14 ] [Guan L.]A College of Chemistry, Fuzhou University, Fuzhou, 350108, China

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Source :

Materials Horizons

ISSN: 2051-6347

Year: 2023

Issue: 9

Volume: 10

Page: 3610-3621

1 2 . 2

JCR@2023

1 2 . 2 0 0

JCR@2023

ESI HC Threshold:49

JCR Journal Grade:1

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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