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author:

Chen, Shuxin (Chen, Shuxin.) [1] | Lin, Jidong (Lin, Jidong.) [2] | Huang, Jie (Huang, Jie.) [3] | Pang, Tao (Pang, Tao.) [4] | Ye, Qingying (Ye, Qingying.) [5] | Zheng, Yuanhui (Zheng, Yuanhui.) [6] (Scholars:郑远辉) | Li, Xiaoyan (Li, Xiaoyan.) [7] | Yu, Yunlong (Yu, Yunlong.) [8] | Zhuang, Bin (Zhuang, Bin.) [9] | Chen, Daqin (Chen, Daqin.) [10]

Indexed by:

EI Scopus SCIE

Abstract:

Robust amorphous glass protected CsPbBr3 (CsPbBr3@glass) perovskite quantum dots (PeQDs) with ultra-pure green emission and superior long-term stability are highly desirable for developing wide-color-gamut liquid crystal displays. However, most of the reported CsPbBr3@glass nanocomposites are subject to low external quantum efficiency (EQE). This work demonstrates that ZrO2 additive has an "accumulation" effect on the borosilicate glass network structure to promote in situ nucleation/growth of PeQDs inside glass rather than self-crystallization. This effect is beneficial in reducing surface defects, improving the quality of PeQDs, and thus boosting radiative recombination of excitons. As a consequence, the as-prepared CsPbBr3@glass shows a record EQE of up to 75% and can pass the accelerated aging tests at 85 degrees C/85% RH for 1000 h and blue light irradiation over 2000 h. Finally, a prototype display using CsPbBr3@glass-based straight-down backlit unit is designed and gains more favorable responses in blind selection tests for its high brightness of 2647 cd m(-2) and high color purity of 88%. The findings will pave the way for realizing the commercial application of CsPbBr3@glass nanocomposite in PeQDs-converted backlit display.

Keyword:

composites glasses light-emitting diodes luminescent materials perovskite quantum dots

Community:

  • [ 1 ] [Chen, Shuxin]Fujian Normal Univ, Coll Phys & Energy, Fuzhou 350117, Fujian, Peoples R China
  • [ 2 ] [Lin, Jidong]Fujian Normal Univ, Coll Phys & Energy, Fuzhou 350117, Fujian, Peoples R China
  • [ 3 ] [Huang, Jie]Fujian Normal Univ, Coll Phys & Energy, Fuzhou 350117, Fujian, Peoples R China
  • [ 4 ] [Ye, Qingying]Fujian Normal Univ, Coll Phys & Energy, Fuzhou 350117, Fujian, Peoples R China
  • [ 5 ] [Zhuang, Bin]Fujian Normal Univ, Coll Phys & Energy, Fuzhou 350117, Fujian, Peoples R China
  • [ 6 ] [Chen, Daqin]Fujian Normal Univ, Coll Phys & Energy, Fuzhou 350117, Fujian, Peoples R China
  • [ 7 ] [Pang, Tao]Huzhou Univ, Coll Sci, Huzhou Key Lab Mat Energy Convers & Storage, Huzhou 313000, Zhejiang, Peoples R China
  • [ 8 ] [Zheng, Yuanhui]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350116, Fujian, Peoples R China
  • [ 9 ] [Chen, Daqin]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350116, Fujian, Peoples R China
  • [ 10 ] [Zheng, Yuanhui]Fuzhou Univ, Coll Chem, Fuzhou 350116, Fujian, Peoples R China
  • [ 11 ] [Li, Xiaoyan]Fujian Jiangxia Univ, Organ Optoelect Engn Res Ctr Fujians Univ, Coll Elect & Informat Sci, Fuzhou 350108, Peoples R China
  • [ 12 ] [Yu, Yunlong]Fujian Jiangxia Univ, Organ Optoelect Engn Res Ctr Fujians Univ, Coll Elect & Informat Sci, Fuzhou 350108, Peoples R China
  • [ 13 ] [Chen, Daqin]Fujian Prov Collaborat Innovat Ctr Adv High Field, Fuzhou 350117, Fujian, Peoples R China
  • [ 14 ] [Chen, Daqin]Fujian Prov Engn Technol Res Ctr Solar Energy Conv, Fuzhou 350117, Fujian, Peoples R China

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Source :

ADVANCED FUNCTIONAL MATERIALS

ISSN: 1616-301X

Year: 2023

Issue: 2

Volume: 34

1 8 . 5

JCR@2023

1 8 . 5 0 0

JCR@2023

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 27

SCOPUS Cited Count: 44

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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