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author：

Lin, Liang (Lin, Liang.) [1] | Yue, Ke (Yue, Ke.) [2] | Xia, Li (Xia, Li.) [3] | Yan, Xiaolin (Yan, Xiaolin.) [4] | Zheng, Hongfei (Zheng, Hongfei.) [5] | Zhang, Yinggan (Zhang, Yinggan.) [6] | Sa, Baisheng (Sa, Baisheng.) [7] | Li, Junjie (Li, Junjie.) [8] | Wang, Laisen (Wang, Laisen.) [9] | Lin, Jie (Lin, Jie.) [10] | Liu, Yujing (Liu, Yujing.) [11] | Wei, Guoying (Wei, Guoying.) [12] | Peng, Dong-Liang (Peng, Dong-Liang.) [13] | Xie, Qingshui (Xie, Qingshui.) [14]

Indexed by：

EI

Abstract：

Irregular　Li　deposition　is　the　major　reason　for　poor　reversibility　and　cycle　instability　in　Li　metal　batteries,　even　leading　to　safety　hazards,　the　causes　of　which　have　been　extensively　explored.　The　structural　disconnection　induced　by　completely　dissolving　Li　in　the　traditional　testing　protocol　is　a　key　factor　accounting　for　irregular　Li　growth　during　the　subsequent　deposition　process.　Herein,　the　critical　role　played　by　the　structural　connectivity　of　electrochemical　Li　reservoir　in　subsequent　Li　deposition　behaviors　is　elucidated　and　a　morphology-performance　correlation　is　established.　The　structural　connection　and　resultant　well-distributed　morphology　of　the　in　situ　electrochemical　Li　reservoir　ensure　efficient　electron　transfer　and　Li+　diffusion　pathway,　finally　leading　to　homogenized　Li　nucleation　and　growth.　Tailoring　the　geometry　of　Li　reservoir　can　improve　the　coulombic　efficiency　and　cyclability　of　anode-free　Li　metal　batteries　by　optimizing　Li　deposition　behavior.　©　2024　Wiley-VCH　GmbH.

Keyword：

Anodes Deposition Morphology

Community：

  • [ 1 ] [Lin, Liang]State Key Lab for Physical Chemistry of Solid Surfaces, Fujian Key Laboratory of Surface and Interface Engineering for High Performance Materials (Xiamen University), College of Materials, Xiamen University, Xiamen; 361005, China
  • [ 2 ] [Yue, Ke]College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou; 310014, China
  • [ 3 ] [Xia, Li]State Key Lab for Physical Chemistry of Solid Surfaces, Fujian Key Laboratory of Surface and Interface Engineering for High Performance Materials (Xiamen University), College of Materials, Xiamen University, Xiamen; 361005, China
  • [ 4 ] [Yan, Xiaolin]State Key Lab for Physical Chemistry of Solid Surfaces, Fujian Key Laboratory of Surface and Interface Engineering for High Performance Materials (Xiamen University), College of Materials, Xiamen University, Xiamen; 361005, China
  • [ 5 ] [Zheng, Hongfei]State Key Lab for Physical Chemistry of Solid Surfaces, Fujian Key Laboratory of Surface and Interface Engineering for High Performance Materials (Xiamen University), College of Materials, Xiamen University, Xiamen; 361005, China
  • [ 6 ] [Zhang, Yinggan]State Key Lab for Physical Chemistry of Solid Surfaces, Fujian Key Laboratory of Surface and Interface Engineering for High Performance Materials (Xiamen University), College of Materials, Xiamen University, Xiamen; 361005, China
  • [ 7 ] [Sa, Baisheng]Multiscale Computational Materials Facility, College of Materials Science and Engineering, Fuzhou University, Fuzhou; 350100, China
  • [ 8 ] [Li, Junjie]School of Applied Mathematics, Xiamen University of Technology, Xiamen; 361024, China
  • [ 9 ] [Wang, Laisen]State Key Lab for Physical Chemistry of Solid Surfaces, Fujian Key Laboratory of Surface and Interface Engineering for High Performance Materials (Xiamen University), College of Materials, Xiamen University, Xiamen; 361005, China
  • [ 10 ] [Lin, Jie]State Key Lab for Physical Chemistry of Solid Surfaces, Fujian Key Laboratory of Surface and Interface Engineering for High Performance Materials (Xiamen University), College of Materials, Xiamen University, Xiamen; 361005, China
  • [ 11 ] [Liu, Yujing]College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou; 310014, China
  • [ 12 ] [Wei, Guoying]College of Materials & Chemistry, China Jiliang University, Hangzhou; 310018, China
  • [ 13 ] [Peng, Dong-Liang]State Key Lab for Physical Chemistry of Solid Surfaces, Fujian Key Laboratory of Surface and Interface Engineering for High Performance Materials (Xiamen University), College of Materials, Xiamen University, Xiamen; 361005, China
  • [ 14 ] [Xie, Qingshui]State Key Lab for Physical Chemistry of Solid Surfaces, Fujian Key Laboratory of Surface and Interface Engineering for High Performance Materials (Xiamen University), College of Materials, Xiamen University, Xiamen; 361005, China

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Angewandte Chemie - International Edition

ISSN： 1433-7851

Year： 2024

Issue： 11

Volume： 63

1 6 . 1 0 0

JCR@2023

CAS Journal Grade：1

Cited Count：

WoS CC Cited Count：

SCOPUS Cited Count： 1

ESI Highly Cited Papers on the List： 0 Unfold All

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Chinese Cited Count：

30 Days PV： 2

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