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author:

Xu, S. (Xu, S..) [1] | Cai, S. (Cai, S..) [2] | Huang, R. (Huang, R..) [3] | Xu, K. (Xu, K..) [4] | Ma, Z. (Ma, Z..) [5] | Fang, L. (Fang, L..) [6] | Zhang, C. (Zhang, C..) [7]

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Scopus

Abstract:

The thermal-oxidative aging of asphalt is extensively researched in recent years. However, the aging behavior of asphalt in salt and water environment receives less attention. A virgin asphalt binder was treated by various coupling conditions of salt and water in this work aiming at understanding the aging behaviors, and then the physical indexes, rheological parameters, chemical structures, four fractions and contact angles of asphalt before and after aging were measured to evaluated the effects of different aging environments on the physicochemical properties of asphalt. Results indicate that the aged asphalt has higher softening point and complex modulus while lower penetration and phase angle in comparison with unaged asphalt, implying the asphalt becomes harder and more brittle after aging. Although asphalt aged in salt and water conditions exhibits similar changes in macro-properties to thermal-oxidative aged asphalt, the analysis of chemical composition indicates that the aging of asphalt under salt and water environment is caused by unique inducements, which can be divided into two parts, that is, separating out of aromatics and saturates from asphalt by combined action of salt out and emulsification, and increasing of asphaltenes and resins caused by oxidation. These two factors work together leading to the change of colloidal structure and finally cause the deteriorate of macro-properties. Besides, the results of contact angle test indicate the increasing polar functional groups resulting from aging enhance hydrophily of asphalt and increase the possibility of water to enter the interior of asphalt, exacerbating the performance degradation of asphalt. © 2024 Elsevier Ltd

Keyword:

Aging evaluation Asphalt Colloidal structure Polar functional groups Salt-water coupling effect

Community:

  • [ 1 ] [Xu S.]College of Civil Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 2 ] [Cai S.]College of Civil Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 3 ] [Huang R.]School of Advanced Manufacturing, Fuzhou University, Fuzhou, 350108, China
  • [ 4 ] [Xu K.]College of Civil Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 5 ] [Ma Z.]Fujian Provincial Transportation Research Institute Co., Ltd., Fuzhou, 350108, China
  • [ 6 ] [Fang L.]College of Civil Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 7 ] [Zhang C.]College of Civil Engineering, Fuzhou University, Fuzhou, 350108, China

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Source :

Fuel

ISSN: 0016-2361

Year: 2024

Volume: 365

6 . 7 0 0

JCR@2023

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 1

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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