A multicomponent triformylphoroglucinol-based covalent organic framework for overall hydrogen peroxide photosynthesis - Details

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Abstract：

A　multicomponent　covalent　organic　framework　(COF-Tfp-BpyDaaq)　integrating　bipyridine　with　diaminoanthraquinone　through　a　triformylphoroglucinol　linkage　was　synthesized　for　the　first　time　as　a　photocatalyst　for　overall　H2O2　photosynthesis.　It　exhibits　enhanced　photo-charge　separation　and　H2O2　production　rate　over　its　two-component　counterparts,　demonstrating　the　pivotal　role　of　multicomponent　synthesis　in　designing　efficient　photocatalysts.　A　multicomponent　covalent　organic　framework　(COF-Tfp-BpyDaaq)　integrating　bipyridine　with　diaminoanthraquinone　through　a　triformylphoroglucinol　linkage　was　synthesized　for　the　first　time　as　a　photocatalyst　for　overall　H2O2　photosynthesis.

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[ 1 ] [Chai, Erchong]Fuzhou Univ, Coll Chem, Fuzhou 350116, Fujian, Peoples R China
[ 2 ] [Huang, Lanting]Fuzhou Univ, Coll Chem, Fuzhou 350116, Fujian, Peoples R China
[ 3 ] [Jiao, Lei]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China
[ 4 ] [Xiao, Zhiwei]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China
[ 5 ] [Zhang, Xiang]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China
[ 6 ] [Wang, Yaobing]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China
[ 7 ] [Jiao, Lei]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Nanomat, State Key Lab Struct Chem, Fuzhou 350002, Fujian, Peoples R China
[ 8 ] [Xiao, Zhiwei]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Nanomat, State Key Lab Struct Chem, Fuzhou 350002, Fujian, Peoples R China
[ 9 ] [Zhang, Xiang]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Nanomat, State Key Lab Struct Chem, Fuzhou 350002, Fujian, Peoples R China
[ 10 ] [Wang, Yaobing]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Nanomat, State Key Lab Struct Chem, Fuzhou 350002, Fujian, Peoples R China
[ 11 ] [Zhang, Xiang]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Fujian, Peoples R China
[ 12 ] [Wang, Yaobing]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Fujian, Peoples R China
[ 13 ] [Jiao, Lei]Univ Chinese Acad Sci, Beijing 100049, Peoples R China
[ 14 ] [Zhang, Xiang]Univ Chinese Acad Sci, Beijing 100049, Peoples R China
[ 15 ] [Wang, Yaobing]Univ Chinese Acad Sci, Beijing 100049, Peoples R China

Reprint 's Address：

[Zhang, Xiang]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China;;[Wang, Yaobing]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China;;[Zhang, Xiang]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Nanomat, State Key Lab Struct Chem, Fuzhou 350002, Fujian, Peoples R China;;[Wang, Yaobing]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Nanomat, State Key Lab Struct Chem, Fuzhou 350002, Fujian, Peoples R China;;[Zhang, Xiang]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Fujian, Peoples R China;;[Wang, Yaobing]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Fujian, Peoples R China;;[Zhang, Xiang]Univ Chinese Acad Sci, Beijing 100049, Peoples R China;;[Wang, Yaobing]Univ Chinese Acad Sci, Beijing 100049, Peoples R China

Email：

zhangxiang@fjirsm.ac.cn |
wangyb@fjirsm.ac.cn

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A multicomponent triformylphoroglucinol-based covalent organic framework for overall hydrogen peroxide photosynthesis
2024，Chemical Communications
A multicomponent triformylphoroglucinol-based covalent organic framework for overall hydrogen peroxide photosynthesis
2024，Chemical Communications

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CHEMICAL COMMUNICATIONS

ISSN： 1359-7345

Year： 2024

Issue： 25

Volume： 60

Page： 3405-3408

4 . 3 0 0

JCR@2023

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ESI Highly Cited Papers on the List： 0 Unfold All

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30 Days PV： 2

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