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author：

Li, Y. (Li, Y..) [1] | Qiu, Z. (Qiu, Z..) [2] | Huang, L. (Huang, L..) [3] | Shen, S. (Shen, S..) [4] | Liu, P. (Liu, P..) [5] | Zhang, H. (Zhang, H..) [6] | Cao, F. (Cao, F..) [7] | He, X. (He, X..) [8] | Zhang, J. (Zhang, J..) [9] | Xia, Y. (Xia, Y..) [10] | Liang, X. (Liang, X..) [11] | Wang, C. (Wang, C..) [12] | Wan, W. (Wan, W..) [13] | Zhang, Y. (Zhang, Y..) [14] | Chen, M. (Chen, M..) [15] | Zhang, W. (Zhang, W..) [16] | Huang, H. (Huang, H..) [17] | Gan, Y. (Gan, Y..) [18] | Xia, X. (Xia, X..) [19]

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Scopus

Abstract：

Silicon　(Si)　is　considered　as　one　of　the　most　promising　anode　materials　for　advanced　lithium-ion　batteries　due　to　its　high　theoretical　capacity,　environmental　friendliness,　and　widespread　availability.　However,　great　challenges　such　as　volumetric　expansion,　limited　ionic/electronic　conductivity　properties　and　complex　manufacturing　processes　hinder　its　practical　applications.　Herein,　a　novel　plasma-enhanced　reduced　graphene　oxide　fibers/Si　(PrGOFs/Si)　composite　anode　is　first　proposed　by　using　wet-spinning　technology　followed　by　plasma-enhanced　reduction　method.　The　PrGOFs　provide　large　space　to　accommodate　the　volume　expansion　of　Si　nanoparticles　(SiNPs)　by　forming　a　flexible　3D　conductive　network.　Compared　to　the　conventional　thermally　reduced　graphene　oxide　fibers/Si　(TrGOFs/Si)　sample,　the　PrGOFs/Si　anodes　demonstrate　higher　conductivity,　specific　surface　area,　and　superior　fabrication　efficiency.　Accordingly,　the　PrGOFs/Si　anodes　exhibit　a　reversible　capacity　of　698.3　mAh/g,　and　maintain　a　specific　capacity　of　602.5　mAh/g　at　a　current　density　of　200　mA/g　after　100　cycles,　superior　to　conventional　TrGOFs/Si　counterparts.　This　research　presents　a　novel　strategy　for　the　preparation　of　high-performance　Si/carbon　anodes　for　energy　storage　applications.　©　2024

Keyword：

Carbon Graphene fibers Li ion batteries Plasma Si anode

Community：

  • [ 1 ] [Li Y.]School of Materials Science & Engineering, Zhejiang University, Hangzhou, 310027, China
  • [ 2 ] [Li Y.]College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou, 310014, China
  • [ 3 ] [Qiu Z.]School of Materials Science & Engineering, Zhejiang University, Hangzhou, 310027, China
  • [ 4 ] [Qiu Z.]College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou, 310014, China
  • [ 5 ] [Huang L.]School of Materials Science & Engineering, Zhejiang University, Hangzhou, 310027, China
  • [ 6 ] [Huang L.]College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou, 310014, China
  • [ 7 ] [Shen S.]School of Materials Science and & Engineering, Zhejiang Sci-Tech University, Hangzhou, 310018, China
  • [ 8 ] [Liu P.]School of Materials Science & Engineering, Zhejiang University, Hangzhou, 310027, China
  • [ 9 ] [Liu P.]College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou, 310014, China
  • [ 10 ] [Zhang H.]School of Materials Science & Engineering, Zhejiang University, Hangzhou, 310027, China
  • [ 11 ] [Cao F.]Department of Engineering Technology, Huzhou College, Huzhou, 313000, China
  • [ 12 ] [He X.]College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou, 310014, China
  • [ 13 ] [Zhang J.]College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou, 310014, China
  • [ 14 ] [Xia Y.]College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou, 310014, China
  • [ 15 ] [Liang X.]Institute of Fundamental and Frontier Science, University of Electronic Science and Technology of China, Chengdu, 611371, China
  • [ 16 ] [Liang X.]Key Laboratory of Engineering Dielectric and Applications (Ministry of Education), School of Electrical and Electronic Engineering, Harbin University of Science and Technology, Harbin, 150080, China
  • [ 17 ] [Wang C.]Zhejiang Academy of Science and Technology for Inspection & Quarantine, Hangzhou, 311215, China
  • [ 18 ] [Wan W.]Zhejiang Academy of Science and Technology for Inspection & Quarantine, Hangzhou, 311215, China
  • [ 19 ] [Zhang Y.]Institute of Fundamental and Frontier Science, University of Electronic Science and Technology of China, Chengdu, 611371, China
  • [ 20 ] [Chen M.]Key Laboratory of Engineering Dielectric and Applications (Ministry of Education), School of Electrical and Electronic Engineering, Harbin University of Science and Technology, Harbin, 150080, China
  • [ 21 ] [Zhang W.]College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou, 310014, China
  • [ 22 ] [Huang H.]College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou, 310014, China
  • [ 23 ] [Gan Y.]College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou, 310014, China
  • [ 24 ] [Xia X.]School of Materials Science & Engineering, Zhejiang University, Hangzhou, 310027, China
  • [ 25 ] [Xia X.]College of Materials Science and Engineering, Zhejiang University of Technology, Hangzhou, 310014, China
  • [ 26 ] [Xia X.]State Key Laboratory of Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou, 350116, China

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Source ：

Chinese Chemical Letters

ISSN： 1001-8417

Year： 2024

Issue： 11

Volume： 35

9 . 4 0 0

JCR@2023

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SCOPUS Cited Count：

ESI Highly Cited Papers on the List： 0 Unfold All

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Chinese Cited Count：

30 Days PV： 2

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