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author：

Yuan, Y. (Yuan, Y..) [1] | Zhang, D.-H. (Zhang, D.-H..) [2] | Li, Q.-H. (Li, Q.-H..) [3] | Chen, S.-M. (Chen, S.-M..) [4] (Scholars：陈淑妹) | He, Y.-P. (He, Y.-P..) [5] | Zhang, J. (Zhang, J..) [6]

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Abstract：

The　integration　of　anionic　Ti4L6　(L　=　embonate)　cages　and　π-conjugated　coordination　cations　into　ordered　structures　can　produce　high-performance　nonlinear　optical　(NLO)　materials.　More　specifically,　by　employing　Ti4L6　cages　for　assembly　with　mixed　N,N-chelated　and　P,P-chelated　type　conjugated　organic　ligands　and　Ag+　ions,　three　cage-based　structures　have　been　synthesized　and　structurally　characterized.　Among　them,　an　ion　pair　structure　with　strong　π-π　accumulation　exhibits　a　significant　third-order　NLO　response,　and　an　excellent　optical　limiting　effect　has　been　experimentally　verified.　This　work　provides　a　promising　material　for　NLO　applications.　©　2024　The　Royal　Society　of　Chemistry.

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  • [ 1 ] [Yuan Y.]College of Chemistry, Fuzhou University, Fujian, Fuzhou, 350108, China
  • [ 2 ] [Yuan Y.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fujian, Fuzhou, 350002, China
  • [ 3 ] [Zhang D.-H.]College of Chemistry, Fuzhou University, Fujian, Fuzhou, 350108, China
  • [ 4 ] [Zhang D.-H.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fujian, Fuzhou, 350002, China
  • [ 5 ] [Li Q.-H.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fujian, Fuzhou, 350002, China
  • [ 6 ] [Chen S.-M.]College of Chemistry, Fuzhou University, Fujian, Fuzhou, 350108, China
  • [ 7 ] [He Y.-P.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fujian, Fuzhou, 350002, China
  • [ 8 ] [Zhang J.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fujian, Fuzhou, 350002, China

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Source ：

Chemical Communications

ISSN： 1359-7345

Year： 2024

Issue： 66

Volume： 60

Page： 8748-8751

4 . 3 0 0

JCR@2023

CAS Journal Grade：3

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ESI Highly Cited Papers on the List： 0 Unfold All

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30 Days PV： 3

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