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author:

Cai, Dandan (Cai, Dandan.) [1] | Zheng, Feng (Zheng, Feng.) [2] | Li, Ying (Li, Ying.) [3] | Zhang, Caizhi (Zhang, Caizhi.) [4] | Qin, Ziwei (Qin, Ziwei.) [5] | Li, Wenxian (Li, Wenxian.) [6] | Liu, Yang (Liu, Yang.) [7] | Li, Aijun (Li, Aijun.) [8] | Zhang, Jiujun (Zhang, Jiujun.) [9]

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Abstract:

Lithium-sulfur batteries (LSBs) are considered next-generation energy storage and conversion solutions owing to their high theoretical specific capacity and the high abundance/low-cost of sulfur-based cathode materials. However, LSBs still encounter significant challenges, including the low conductivities of sulfur-based materials, severe volumetric expansion of sulfur during the discharge process, and the persistent 'shuttle effect' of polysulfides. In recent years, a tremendous amount of research has been conducted to address the above challenges by developing coating and compositing materials and corresponding fabrication strategies for sulfur-based cathode materials. In this study, the surface coating, compositing materials, and fabrication methodologies of LSB cathodes are comprehensively reviewed in terms of advanced materials, structure/component characterization, functional mechanisms, and performance validation. Some technical challenges are analyzed in detail, and possible future research directions are proposed to overcome the challenges toward practical applications of lithium-sulfur batteries. © 2024 Wiley-VCH GmbH.

Keyword:

Cathodes Coatings Lithium batteries Lithium sulfur batteries

Community:

  • [ 1 ] [Cai, Dandan]College of Sciences, Shanghai University, Shanghai; 200444, China
  • [ 2 ] [Zheng, Feng]College of Sciences, Shanghai University, Shanghai; 200444, China
  • [ 3 ] [Li, Ying]School of Materials Science and Engineering, Shanghai University, Shanghai; 200072, China
  • [ 4 ] [Zhang, Caizhi]College of Mechanical and Vehicle Engineering, The State Key Laboratory of Mechanical Transmissions, Chongqing Automotive Collaborative Innovation Center, Chongqing University, Chongqing; 400044, China
  • [ 5 ] [Qin, Ziwei]School of Materials Science and Engineering, Shanghai University, Shanghai; 200072, China
  • [ 6 ] [Qin, Ziwei]Shaoxing Institute of Technology, Shanghai University, Zhejiang, Shaoxing; 312000, China
  • [ 7 ] [Li, Wenxian]School of Materials Science and Engineering, Shanghai University, Shanghai; 200072, China
  • [ 8 ] [Li, Wenxian]School of Materials Science and Engineering/Materials and Manufacturing Futures Institute, The University of New South Wales, Sydney; NSW; 2052, Australia
  • [ 9 ] [Liu, Yang]College of Sciences, Shanghai University, Shanghai; 200444, China
  • [ 10 ] [Liu, Yang]Shaoxing Institute of Technology, Shanghai University, Zhejiang, Shaoxing; 312000, China
  • [ 11 ] [Li, Aijun]Shaoxing Institute of Technology, Shanghai University, Zhejiang, Shaoxing; 312000, China
  • [ 12 ] [Zhang, Jiujun]College of Sciences, Shanghai University, Shanghai; 200444, China
  • [ 13 ] [Zhang, Jiujun]College of Materials Science and Engineering, Fuzhou University, Fujian; 350108, China

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Source :

Chemistry - An Asian Journal

ISSN: 1861-4728

Year: 2024

Issue: 17

Volume: 19

3 . 5 0 0

JCR@2023

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 2

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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