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author:

Ma, Bowen (Ma, Bowen.) [1] | Yu, Fangyuan (Yu, Fangyuan.) [2] | Zhou, Ping (Zhou, Ping.) [3] | Wu, Xiao (Wu, Xiao.) [4] (Scholars:吴啸) | Zhao, Chunlin (Zhao, Chunlin.) [5] (Scholars:赵纯林) | Lin, Cong (Lin, Cong.) [6] (Scholars:林枞) | Gao, Min (Gao, Min.) [7] (Scholars:高旻) | Lin, Tengfei (Lin, Tengfei.) [8] (Scholars:林腾飞) | Sa, Baisheng (Sa, Baisheng.) [9] (Scholars:萨百晟)

Abstract:

High optical transmittance (T%) has always been an important indicator of transparent-ferroelectric ceramics for optoelectronic coupling. However, the pathway of pursuing high transparency has been at the experimental trial-and-error stage over the past decades, manifesting major drawbacks of being time-consuming and resource-wasting. The present work introduces a machine learning (ML) accelerated development of highly transparent-ferroelectrics by taking potassium-sodium niobate (KNN)-based ceramics as the model material. It is highlighted that by using a small data set of 118 sample data and four key features, we predict the T% of un-synthesized KNN-based ceramics and evaluate the importance of key features. Meanwhile, the screened (K0.5Na0.5)(0.956)Tb0.004Ba0.04NbO3 ceramics were successfully realized by the conventional solid-state synthesis, and the experimental measured T% is in full agreement with the predicted results, exhibiting a satisfactory high T% of similar to 78% at 800 nm. In addition, ML is also used to explore the best experimental parameters, and the prediction results of T% are particularly sensitive to changes in sintering temperature (ST). Eventually, the predicted optimal ST is highly consistent with the experimental one. This study constructs a new avenue for exploring high T% ferroelectric KNN ceramics based on ML, ascertaining optimal process parameters, and guiding the development of other transparent-ferroelectrics in optoelectronic fields.

Keyword:

KNN-based ceramics Machine learning sintering temperature transmittance

Community:

  • [ 1 ] [Ma, Bowen]Fuzhou Univ, Coll Mat Sci & Engn, 2 Xueyuan Rd, Fuzhou 350108, Fujian, Peoples R China
  • [ 2 ] [Yu, Fangyuan]Fuzhou Univ, Coll Mat Sci & Engn, 2 Xueyuan Rd, Fuzhou 350108, Fujian, Peoples R China
  • [ 3 ] [Zhou, Ping]Fuzhou Univ, Coll Mat Sci & Engn, 2 Xueyuan Rd, Fuzhou 350108, Fujian, Peoples R China
  • [ 4 ] [Wu, Xiao]Fuzhou Univ, Coll Mat Sci & Engn, 2 Xueyuan Rd, Fuzhou 350108, Fujian, Peoples R China
  • [ 5 ] [Zhao, Chunlin]Fuzhou Univ, Coll Mat Sci & Engn, 2 Xueyuan Rd, Fuzhou 350108, Fujian, Peoples R China
  • [ 6 ] [Lin, Cong]Fuzhou Univ, Coll Mat Sci & Engn, 2 Xueyuan Rd, Fuzhou 350108, Fujian, Peoples R China
  • [ 7 ] [Gao, Min]Fuzhou Univ, Coll Mat Sci & Engn, 2 Xueyuan Rd, Fuzhou 350108, Fujian, Peoples R China
  • [ 8 ] [Lin, Tengfei]Fuzhou Univ, Coll Mat Sci & Engn, 2 Xueyuan Rd, Fuzhou 350108, Fujian, Peoples R China
  • [ 9 ] [Sa, Baisheng]Fuzhou Univ, Coll Mat Sci & Engn, 2 Xueyuan Rd, Fuzhou 350108, Fujian, Peoples R China

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Source :

JOURNAL OF MATERIALS INFORMATICS

Year: 2023

Issue: 2

Volume: 3

Cited Count:

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ESI Highly Cited Papers on the List: 0 Unfold All

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Chinese Cited Count:

30 Days PV: 6

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