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author:

Yan, Jun (Yan, Jun.) [1] | Cui, Tao (Cui, Tao.) [2] | Su, Qin (Su, Qin.) [3] | Wu, Haidi (Wu, Haidi.) [4] | Xiao, Wei (Xiao, Wei.) [5] | Ye, Liping (Ye, Liping.) [6] | Hou, Suyang (Hou, Suyang.) [7] | Xue, Huaiguo (Xue, Huaiguo.) [8] | Shi, Yongqian (Shi, Yongqian.) [9] (Scholars:施永乾) | Tang, Longcheng (Tang, Longcheng.) [10] | Song, Pingan (Song, Pingan.) [11] | Gao, Jiefeng (Gao, Jiefeng.) [12]

Indexed by:

EI Scopus SCIE

Abstract:

Recently, solar-driven interfacial evaporation (SDIE) has been developed quickly for low-cost and sustainable seawater desalination, but addressing the conflict between a high evaporation rate and salt rejection during SDIE is still challenging. Here, a spatial confinement strategy is proposed to prepare the gel composite solar evaporator (SCE) by loading one thin hydrogel layer onto the skeleton of a carbon aerogel. The SCE retains the hierarchically porous structure of carbon aerogels with an optimized water supply induced by dual-driven forces (capillary effects and osmotic pressure) and takes advantage of both aerogels and hydrogels, which can gain energy from air and reduce water enthalpy. The SCE has a high evaporation rate (up to 4.23 kg m-2 h-1 under one sun) and excellent salt rejection performance and can maintain structural integrity after long-term evaporation even at high salinities. The SDIE behavior, including heat distribution, water transport, and salt ion distribution, is investigated by combining theoretical simulations and experimental results. This work provides new inspiration and a theoretical basis for the development of high-performance interfacial evaporators. The spatially confined hydrogel-modified interfacial evaporator (SCE) is prepared in this study. Dual-driven forces for water transportation of SCE including capillary effect and osmotic pressure ensure sufficient water supply for continuous evaporation up to 4.23 kg m-2 h-1 under one sun and excellent salt rejection performance that it can work in 20 wt.% saltwater stably for the long term. image

Keyword:

carbon aerogel hydrogel interfacial evaporation solar steam generation

Community:

  • [ 1 ] [Yan, Jun]Yangzhou Univ, Sch Chem & Chem Engn, Yangzhou 225002, Peoples R China
  • [ 2 ] [Cui, Tao]Yangzhou Univ, Sch Chem & Chem Engn, Yangzhou 225002, Peoples R China
  • [ 3 ] [Su, Qin]Yangzhou Univ, Sch Chem & Chem Engn, Yangzhou 225002, Peoples R China
  • [ 4 ] [Wu, Haidi]Yangzhou Univ, Sch Chem & Chem Engn, Yangzhou 225002, Peoples R China
  • [ 5 ] [Xiao, Wei]Yangzhou Univ, Sch Chem & Chem Engn, Yangzhou 225002, Peoples R China
  • [ 6 ] [Ye, Liping]Yangzhou Univ, Sch Chem & Chem Engn, Yangzhou 225002, Peoples R China
  • [ 7 ] [Hou, Suyang]Yangzhou Univ, Sch Chem & Chem Engn, Yangzhou 225002, Peoples R China
  • [ 8 ] [Xue, Huaiguo]Yangzhou Univ, Sch Chem & Chem Engn, Yangzhou 225002, Peoples R China
  • [ 9 ] [Gao, Jiefeng]Yangzhou Univ, Sch Chem & Chem Engn, Yangzhou 225002, Peoples R China
  • [ 10 ] [Shi, Yongqian]Fuzhou Univ, Coll Environm & Safety Engn, Fuzhou 350116, Peoples R China
  • [ 11 ] [Tang, Longcheng]Hangzhou Normal Univ, Coll Mat Chem & Chem Engn, Key Lab Organosilicon Chem & Mat Technol, MoE,Key Lab Silicone Mat Technol Zhejiang Prov, Hangzhou 311121, Peoples R China
  • [ 12 ] [Song, Pingan]Univ Southern Queensland, Ctr Future Mat, Springfield Campus, Springfield, Qld 4300, Australia

Reprint 's Address:

  • [Xue, Huaiguo]Yangzhou Univ, Sch Chem & Chem Engn, Yangzhou 225002, Peoples R China;;[Gao, Jiefeng]Yangzhou Univ, Sch Chem & Chem Engn, Yangzhou 225002, Peoples R China;;

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Source :

ADVANCED SCIENCE

Year: 2024

Issue: 41

Volume: 11

1 4 . 3 0 0

JCR@2023

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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