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author:

Wang, Y. (Wang, Y..) [1] | Zhang, J. (Zhang, J..) [2] | Wu, X. (Wu, X..) [3] | Wang, S. (Wang, S..) [4] | Anpo, M. (Anpo, M..) [5] | Fang, Y. (Fang, Y..) [6]

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Abstract:

Solar-induced water oxidation reaction (WOR) for oxygen evolution is a critical step in the transformation of Earth's atmosphere from a reducing to an oxidation one during its primordial stages. WOR is also associated with important reduction reactions, such as oxygen reduction reaction (ORR), which leads to the production of hydrogen peroxide (H2O2). These transitions are instrumental in the emergence and evolution of life. In this study, transition metals were loaded onto nitrogen-doped carbon (NDC) prepared under the primitive Earth's atmospheric conditions. These metal-loaded NDC samples were found to catalyze both WOR and ORR under light illumination. The chemical pathways initiated by the pristine and metal-loaded NDC were investigated. This study provides valuable insights into potential mechanisms relevant to the early evolution of our planet. © 2024

Keyword:

Chemical vapor deposition Nitrogen-doped carbon Oxygen reduction reaction Photocatalysis Water oxidation reaction

Community:

  • [ 1 ] [Wang Y.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350116, China
  • [ 2 ] [Zhang J.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350116, China
  • [ 3 ] [Wu X.]Sino-UK International Joint Laboratory on Photocatalysis for Clean Energy and Advanced Chemicals & Materials, Fuzhou University, Fuzhou, 350108, China
  • [ 4 ] [Wu X.]Department of Chemistry and Materials Innovation Factory, University of Liverpool, Liverpool, L69 7ZD, United Kingdom
  • [ 5 ] [Wang S.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350116, China
  • [ 6 ] [Anpo M.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350116, China
  • [ 7 ] [Fang Y.]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou, 350116, China
  • [ 8 ] [Fang Y.]Sino-UK International Joint Laboratory on Photocatalysis for Clean Energy and Advanced Chemicals & Materials, Fuzhou University, Fuzhou, 350108, China

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Source :

Chinese Chemical Letters

ISSN: 1001-8417

Year: 2025

Issue: 2

Volume: 36

9 . 4 0 0

JCR@2023

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SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

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Chinese Cited Count:

30 Days PV: 1

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