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author:

Guoxi Xiao (Guoxi Xiao.) [1] | Xiaoling Chen (Xiaoling Chen.) [2] | Tiesen Li (Tiesen Li.) [3] (Scholars:李铁森) | Chan Wang (Chan Wang.) [4] (Scholars:王婵) | Qingyan Cui (Qingyan Cui.) [5] (Scholars:崔勍焱) | Yuanyuan Yue (Yuanyuan Yue.) [6] (Scholars:岳源源)

Abstract:

The development of sustainable techniques to produce high-performance zeolite is essential to achieve green production in industry.Herein,we report an eco-friendly route to synthesizing hierarchical Beta zeolite from kaolinite and recycled mother liquor.The results reveal that the unutilized species(such as silicon species and Na+)in mother liquor stayed in a stable concentration during eleven recycled experiments.Moreover,the syn-thesized Beta zeolites still have comparable physicochemical properties and catalytic performance in the esteri-fication of levulinic acid with ethanol over the initial zeolite although eleven recycled experiments.Life cycle assessment exhibits that the synthesis of Beta zeolite with recycled mother liquor can reduce global warming potential by 23%and resource depletion-water use by 36%compared to that without recycled mother liquor.This quantitatively demonstrates that the approach proposed in this work is really a sustainable one,extremely increasing the utilization efficiency of raw materials and decreasing the environmental burden.

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  • [ 1 ] [Qingyan Cui]National Engineering Research Center of Chemical Fertilizer Catalyst,College of Chemical Engineering,Fuzhou University,Fuzhou,350002,China;Qingyuan Innovation Laboratory,Quanzhou,362801,China
  • [ 2 ] [Chan Wang]National Engineering Research Center of Chemical Fertilizer Catalyst,College of Chemical Engineering,Fuzhou University,Fuzhou,350002,China;Qingyuan Innovation Laboratory,Quanzhou,362801,China
  • [ 3 ] [Guoxi Xiao]National Engineering Research Center of Chemical Fertilizer Catalyst,College of Chemical Engineering,Fuzhou University,Fuzhou,350002,China;Qingyuan Innovation Laboratory,Quanzhou,362801,China
  • [ 4 ] [Tiesen Li]National Engineering Research Center of Chemical Fertilizer Catalyst,College of Chemical Engineering,Fuzhou University,Fuzhou,350002,China;Qingyuan Innovation Laboratory,Quanzhou,362801,China
  • [ 5 ] [Yuanyuan Yue]National Engineering Research Center of Chemical Fertilizer Catalyst,College of Chemical Engineering,Fuzhou University,Fuzhou,350002,China;Qingyuan Innovation Laboratory,Quanzhou,362801,China
  • [ 6 ] [Xiaoling Chen]福州大学

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绿色化学工程(英文)

Year: 2024

Issue: 4

Volume: 5

Page: 501-510

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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