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author:

Zhang, Yong-Hui (Zhang, Yong-Hui.) [1] | Wang, Zuo-Bei (Wang, Zuo-Bei.) [2] | Adeoye, Adenike Bernice Eloise (Adeoye, Adenike Bernice Eloise.) [3] | Wang, Yi-Fan (Wang, Yi-Fan.) [4] | Huang, You-Gui (Huang, You-Gui.) [5] | Ye, Xin (Ye, Xin.) [6] | Wang, Wei (Wang, Wei.) [7]

Indexed by:

EI Scopus SCIE

Abstract:

Lanthanum (La) adsorbents are highly effective for phosphorus removal but are constrained by their high reagent cost because of their La content. By exploiting the similarity in ionic sizes between Ca2+ and La3+, we develop a low-cost composite adsorbent LCCa-5@Dia by doping La2(CO3)3 & sdot;8H2O with Ca2+. Our results indicate that the slow addition of NaHCO3 during the synthetic process facilitates the incorporation of Ca2+ into the La2(CO3)3 & sdot;8H2O lattice, leading to an adsorption behavior nearly identical to that of the undoped adsorbents. LCCa-5@Dia demonstrates a high adsorption capacity of 60.04 mg P/g, with stable performance across a pH range of 3 to 11. Its adsorption property also exhibits excellent stability under the interference of solution pH and competing ions. Materials characterization reveals that the adsorption occurs through electrostatic attraction and ligand exchange. In continuous column-adsorption experiments, the LCCa-5@Dia adsorbent treats up to 4000 bed volumes of simulated low concentration wastewater (1.7-2.7 mg P/L). This translates to a treatment cost as low as $0.0211/m3. Meanwhile, the adsorbent also maintains over 80 % of the adsorption capacity after three regeneration cycles. The excellent performance and low treatment cost of the calcium-doped lanthanum carbonate adsorbents highlight its practical potential in treating low concentration wastewater.

Keyword:

Adsorbent Adsorption mechanism Calcium carbonate Lanthanum carbonate Low concentration phosphate removal

Community:

  • [ 1 ] [Zhang, Yong-Hui]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China
  • [ 2 ] [Wang, Zuo-Bei]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China
  • [ 3 ] [Wang, Yi-Fan]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China
  • [ 4 ] [Huang, You-Gui]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China
  • [ 5 ] [Wang, Wei]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China
  • [ 6 ] [Zhang, Yong-Hui]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Nanomat, Fuzhou 350002, Fujian, Peoples R China
  • [ 7 ] [Wang, Zuo-Bei]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Nanomat, Fuzhou 350002, Fujian, Peoples R China
  • [ 8 ] [Wang, Yi-Fan]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Nanomat, Fuzhou 350002, Fujian, Peoples R China
  • [ 9 ] [Huang, You-Gui]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Nanomat, Fuzhou 350002, Fujian, Peoples R China
  • [ 10 ] [Wang, Wei]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Nanomat, Fuzhou 350002, Fujian, Peoples R China
  • [ 11 ] [Zhang, Yong-Hui]Chinese Acad Sci, Xiamen Inst Rare Earth Mat, Haixi Inst, Xiamen Key Lab Rare Earth Photoelect Funct Mat, Xiamen 361021, Fujian, Peoples R China
  • [ 12 ] [Wang, Zuo-Bei]Chinese Acad Sci, Xiamen Inst Rare Earth Mat, Haixi Inst, Xiamen Key Lab Rare Earth Photoelect Funct Mat, Xiamen 361021, Fujian, Peoples R China
  • [ 13 ] [Wang, Yi-Fan]Chinese Acad Sci, Xiamen Inst Rare Earth Mat, Haixi Inst, Xiamen Key Lab Rare Earth Photoelect Funct Mat, Xiamen 361021, Fujian, Peoples R China
  • [ 14 ] [Huang, You-Gui]Chinese Acad Sci, Xiamen Inst Rare Earth Mat, Haixi Inst, Xiamen Key Lab Rare Earth Photoelect Funct Mat, Xiamen 361021, Fujian, Peoples R China
  • [ 15 ] [Ye, Xin]Chinese Acad Sci, Xiamen Inst Rare Earth Mat, Haixi Inst, Xiamen Key Lab Rare Earth Photoelect Funct Mat, Xiamen 361021, Fujian, Peoples R China
  • [ 16 ] [Wang, Wei]Chinese Acad Sci, Xiamen Inst Rare Earth Mat, Haixi Inst, Xiamen Key Lab Rare Earth Photoelect Funct Mat, Xiamen 361021, Fujian, Peoples R China
  • [ 17 ] [Zhang, Yong-Hui]Univ Chinese Acad Sci, Beijing 100049, Peoples R China
  • [ 18 ] [Huang, You-Gui]Univ Chinese Acad Sci, Beijing 100049, Peoples R China
  • [ 19 ] [Wang, Wei]Univ Chinese Acad Sci, Beijing 100049, Peoples R China
  • [ 20 ] [Adeoye, Adenike Bernice Eloise]Chinese Acad Sci, Key Lab Urban Pollutant Convers, Inst Urban Environm, Xiamen 361021, Peoples R China
  • [ 21 ] [Ye, Xin]Chinese Acad Sci, Key Lab Urban Pollutant Convers, Inst Urban Environm, Xiamen 361021, Peoples R China
  • [ 22 ] [Wang, Yi-Fan]Fuzhou Univ, Coll Chem, Fuzhou 350108, Fujian, Peoples R China
  • [ 23 ] [Wang, Wei]Fuzhou Univ, Coll Chem, Fuzhou 350108, Fujian, Peoples R China

Reprint 's Address:

  • [Wang, Wei]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China;;[Wang, Wei]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Nanomat, Fuzhou 350002, Fujian, Peoples R China;;[Ye, Xin]Chinese Acad Sci, Xiamen Inst Rare Earth Mat, Haixi Inst, Xiamen Key Lab Rare Earth Photoelect Funct Mat, Xiamen 361021, Fujian, Peoples R China;;[Wang, Wei]Chinese Acad Sci, Xiamen Inst Rare Earth Mat, Haixi Inst, Xiamen Key Lab Rare Earth Photoelect Funct Mat, Xiamen 361021, Fujian, Peoples R China

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Source :

SEPARATION AND PURIFICATION TECHNOLOGY

ISSN: 1383-5866

Year: 2025

Volume: 360

8 . 2 0 0

JCR@2023

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 6

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