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author：

Chen, H. (Chen, H..) [1] | Song, J. (Song, J..) [2] | Liao, Y. (Liao, Y..) [3] | Weng, Y. (Weng, Y..) [4] | You, H. (You, H..) [5] | Long, X. (Long, X..) [6] | Liu, D. (Liu, D..) [7] | Zhang, J. (Zhang, J..) [8] | Luo, J.-L. (Luo, J.-L..) [9] | Fu, X.-Z. (Fu, X.-Z..) [10]

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Scopus

Abstract：

It　remains　challenges　for　conversion　of　CO2-derived　alcohol　into　electrical　energy　while　without　CO2　greenhouse　gases　emission.　Herein,　a　novel　sustainable　CO2-emssion　free　direct　alcohol　fuel　cell　(DAFC)　is　developed　by　using　Pt-Au/nickel　mesh　anode　with　highly　selective　electrocatalytic　oxidation　of　alcohol　to　acetate　value-added　chemicals.　The　DAFC　demonstrate　a　peak　power　density　of　72.9　mW　cm−2　and　simultaneously　co-synthesis　25　mol　of　acetate　per　1　kWh　of　electrical　energy　output.　This　study　realizes　the　clean　and　efficient　use　of　CO2-derived　carbon-based　fuels,　highly　selective　synthesis　of　acetate　under　mild　conditions　and　generating　electricity　while　without　CO2　greenhouse　gases　emission,　realizing　a　“negative　carbon”　cycle　for　sustainable　development.　©　2025

Keyword：

CO2-Emission Free Direct Alcohol Fuel Cell Negative Carbon Cycle Selective Oxidation Value-Added Products

Community：

  • [ 1 ] [Chen H.]Shenzhen Key Laboratory of Energy Electrocatalytic Materials, Guangdong Provincial Key Laboratory of New Energy Materials Service Safety, College of Materials Science and Engineering, Shenzhen University, Shenzhen, 518055, China
  • [ 2 ] [Chen H.]College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, 361005, China
  • [ 3 ] [Song J.]Shenzhen Key Laboratory of Energy Electrocatalytic Materials, Guangdong Provincial Key Laboratory of New Energy Materials Service Safety, College of Materials Science and Engineering, Shenzhen University, Shenzhen, 518055, China
  • [ 4 ] [Song J.]College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, 361005, China
  • [ 5 ] [Liao Y.]Shenzhen Key Laboratory of Energy Electrocatalytic Materials, Guangdong Provincial Key Laboratory of New Energy Materials Service Safety, College of Materials Science and Engineering, Shenzhen University, Shenzhen, 518055, China
  • [ 6 ] [Weng Y.]Shenzhen Key Laboratory of Energy Electrocatalytic Materials, Guangdong Provincial Key Laboratory of New Energy Materials Service Safety, College of Materials Science and Engineering, Shenzhen University, Shenzhen, 518055, China
  • [ 7 ] [You H.]Shenzhen Key Laboratory of Energy Electrocatalytic Materials, Guangdong Provincial Key Laboratory of New Energy Materials Service Safety, College of Materials Science and Engineering, Shenzhen University, Shenzhen, 518055, China
  • [ 8 ] [Long X.]Shenzhen Key Laboratory of Energy Electrocatalytic Materials, Guangdong Provincial Key Laboratory of New Energy Materials Service Safety, College of Materials Science and Engineering, Shenzhen University, Shenzhen, 518055, China
  • [ 9 ] [Liu D.]Shenzhen Key Laboratory of Energy Electrocatalytic Materials, Guangdong Provincial Key Laboratory of New Energy Materials Service Safety, College of Materials Science and Engineering, Shenzhen University, Shenzhen, 518055, China
  • [ 10 ] [Zhang J.]College of Materials Science and Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 11 ] [Luo J.-L.]Shenzhen Key Laboratory of Energy Electrocatalytic Materials, Guangdong Provincial Key Laboratory of New Energy Materials Service Safety, College of Materials Science and Engineering, Shenzhen University, Shenzhen, 518055, China
  • [ 12 ] [Fu X.-Z.]Shenzhen Key Laboratory of Energy Electrocatalytic Materials, Guangdong Provincial Key Laboratory of New Energy Materials Service Safety, College of Materials Science and Engineering, Shenzhen University, Shenzhen, 518055, China

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Source ：

Nano Energy

ISSN： 2211-2855

Year： 2025

Volume： 138

1 6 . 8 0 0

JCR@2023

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ESI Highly Cited Papers on the List： 0 Unfold All

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30 Days PV： 1

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