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author:

Su, Haobin (Su, Haobin.) [1] | Zheng, Shiyun (Zheng, Shiyun.) [2] | Wang, Ning (Wang, Ning.) [3] | Zhu, Guofeng (Zhu, Guofeng.) [4] | Ju, Xuewei (Ju, Xuewei.) [5] | Huang, Feng (Huang, Feng.) [6] | Cao, Yiming (Cao, Yiming.) [7] | Wang, Xiangfeng (Wang, Xiangfeng.) [8] (Scholars:王向峰)

Indexed by:

EI SCIE

Abstract:

Rare-earth orthoferrites (RFeO3) have received significant attention due to their intricate magnetic interactions and potential applications in ultrafast spintronic devices. Among them, DyFeO3 exhibits rich magnetic phase transitions driven by the interplay between Fe3+ and Dy3+ sublattices. Previous studies mainly focused on temperature-induced spin reorientation near the Morin temperature (T-M similar to 50 K), but there has been limited exploration of magnetic phase behavior under external fields above T-M. This work aims to systematically investigate the temperature- and magnetic-field-dependent magneto-dynamic properties of a-cut DyFeO3 single crystals, with an emphasis on identifying novel phase transitions and elucidating the underlying mechanisms involving Fe3+-Dy3+ anisotropic exchange interactions. High-quality a-cut DyFeO3 single crystals are grown using the optical floating zone method and characterized by X-ray diffraction (XRD) and Laue diffraction. Time-domain terahertz spectroscopy (THz-TDS) coupled with a superconducting magnet (0-7 T, 1.6-300 K) is employed to probe the ferromagnetic resonance (FM) and antiferromagnetic resonance (AFMR) modes. By analyzing the frequency trends in the spectra, the response of internal magnetic moments to external stimuli can be inferred. In the zero magnetic field experiment, it is found that the temperature induced spin reorientation (Gamma(4)->Gamma(1)) occurs at Morin temperature (similar to 50 K) with temperature decreasing. A broadband electromagnetic absorption (0.45-0.9 THz) occurs below 4 K, which is attributed to electromagnons activated by broken inversion symmetry in the Dy3+ antiferromagnetic state. Above the Morin temperature, the absorption spectra of the sample are measured at constant temperatures (70, 77, 90, 100 K) and magnetic fields ranging from 0 to 7 T. The experimental results show that with the increase of magnetic field, a new magnetic phase transition occurs (Gamma(4) -> Gamma(24) -> Gamma(2) -> Gamma(24) -> Gamma(2)), and the critical magnetic field of the phase transition varies with temperature. The phase transitions arise from the competition between external magnetic fields and internal effective fields generated by anisotropic Fe3+-Dy3+ exchange. These findings contribute to the further understanding of the magnetoelectric effects in RFeO3 systems and provide a roadmap for using field-tunable phase transitions to design spin-based devices.

Keyword:

magnetic phase transition magnetic resonance rare-earth orthoferrite terahertz

Community:

  • [ 1 ] [Su, Haobin]Fuzhou Univ, Sch Mech Engn & Automat, Fujian Prov Key Lab Terahertz Funct Devices & Inte, Fuzhou 350108, Peoples R China
  • [ 2 ] [Zhu, Guofeng]Fuzhou Univ, Sch Mech Engn & Automat, Fujian Prov Key Lab Terahertz Funct Devices & Inte, Fuzhou 350108, Peoples R China
  • [ 3 ] [Ju, Xuewei]Fuzhou Univ, Sch Mech Engn & Automat, Fujian Prov Key Lab Terahertz Funct Devices & Inte, Fuzhou 350108, Peoples R China
  • [ 4 ] [Huang, Feng]Fuzhou Univ, Sch Mech Engn & Automat, Fujian Prov Key Lab Terahertz Funct Devices & Inte, Fuzhou 350108, Peoples R China
  • [ 5 ] [Wang, Xiangfeng]Fuzhou Univ, Sch Mech Engn & Automat, Fujian Prov Key Lab Terahertz Funct Devices & Inte, Fuzhou 350108, Peoples R China
  • [ 6 ] [Zheng, Shiyun]Qujing Normal Univ, Sch Phys & Elect Engn, Qujing 655011, Peoples R China
  • [ 7 ] [Cao, Yiming]Qujing Normal Univ, Sch Phys & Elect Engn, Qujing 655011, Peoples R China
  • [ 8 ] [Wang, Ning]Xiamen Univ, Pen Tung Sah Inst Micro Nano Sci & Technol, Xiamen 361102, Peoples R China

Reprint 's Address:

  • 王向峰

    [Ju, Xuewei]Fuzhou Univ, Sch Mech Engn & Automat, Fujian Prov Key Lab Terahertz Funct Devices & Inte, Fuzhou 350108, Peoples R China;;[Wang, Xiangfeng]Fuzhou Univ, Sch Mech Engn & Automat, Fujian Prov Key Lab Terahertz Funct Devices & Inte, Fuzhou 350108, Peoples R China;;[Cao, Yiming]Qujing Normal Univ, Sch Phys & Elect Engn, Qujing 655011, Peoples R China

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Source :

ACTA PHYSICA SINICA

ISSN: 1000-3290

Year: 2025

Issue: 8

Volume: 74

0 . 8 0 0

JCR@2023

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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