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author:

Hu, Fen (Hu, Fen.) [1] | Chen, Kai (Chen, Kai.) [2] | Lu, Zhiwen (Lu, Zhiwen.) [3] | Gao, Jiyuan (Gao, Jiyuan.) [4] | Lan, Senchen (Lan, Senchen.) [5] | Chen, Junxiang (Chen, Junxiang.) [6] | Ci, Suqin (Ci, Suqin.) [7] | Wen, Zhenhai (Wen, Zhenhai.) [8]

Indexed by:

SCIE

Abstract:

Formaldehyde (HCHO), a promising yet challenging hydrogen carrier, offers a unique opportunity for efficient hydrogen generation through electro-oxidation, simultaneously eliminating harmful HCHO and contributing to environmental sustainability. This study rises to the challenge by pioneering a hybrid acid/alkali formaldehyde hydrogen production fuel cell (h-AAFHFC), an integrated system that integrates anodic partial electro-reforming of aldehydes at low potential with the cathodic hydrogen evolution reaction (HER). The device introduces a new self-powered paradigm for hydrogen generation, driven by electrochemical neutralization energy (ENE), featuring high Faradaic efficiency for hydrogen production, co-generation of electricity, and HCOOH. The h-AAFHFC attains an open-circuit voltage (OCV) of 1.11 V and a peak power density of 94 mW cm-2, enabling simultaneous hydrogen production at both electrodes with an extraordinary Faradaic efficiency of approximately 200%. This breakthrough marks a transformative shift, moving from traditional electricity-driven systems to self-sustaining H2 generation. Our work demonstrates a promising pathway for sustainable hydrogen production, advancing the potential of clean hydrogen energy technologies.

Keyword:

Electrocatalysis Electro-reforming of aldehydes High Faradaic efficiency Hybrid acid/alkali fuel cell Self-powered hydrogen generation

Community:

  • [ 1 ] [Hu, Fen]Chinese Acad Sci, State Key Lab Struct Chem, Fuzhou 350002, Fujian, Peoples R China
  • [ 2 ] [Chen, Kai]Chinese Acad Sci, State Key Lab Struct Chem, Fuzhou 350002, Fujian, Peoples R China
  • [ 3 ] [Lu, Zhiwen]Chinese Acad Sci, State Key Lab Struct Chem, Fuzhou 350002, Fujian, Peoples R China
  • [ 4 ] [Gao, Jiyuan]Chinese Acad Sci, State Key Lab Struct Chem, Fuzhou 350002, Fujian, Peoples R China
  • [ 5 ] [Chen, Junxiang]Chinese Acad Sci, State Key Lab Struct Chem, Fuzhou 350002, Fujian, Peoples R China
  • [ 6 ] [Wen, Zhenhai]Chinese Acad Sci, State Key Lab Struct Chem, Fuzhou 350002, Fujian, Peoples R China
  • [ 7 ] [Hu, Fen]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Mat & Tech Hydrogen Energy, Fuzhou 350002, Fujian, Peoples R China
  • [ 8 ] [Chen, Kai]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Mat & Tech Hydrogen Energy, Fuzhou 350002, Fujian, Peoples R China
  • [ 9 ] [Lu, Zhiwen]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Mat & Tech Hydrogen Energy, Fuzhou 350002, Fujian, Peoples R China
  • [ 10 ] [Gao, Jiyuan]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Mat & Tech Hydrogen Energy, Fuzhou 350002, Fujian, Peoples R China
  • [ 11 ] [Chen, Junxiang]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Mat & Tech Hydrogen Energy, Fuzhou 350002, Fujian, Peoples R China
  • [ 12 ] [Wen, Zhenhai]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Mat & Tech Hydrogen Energy, Fuzhou 350002, Fujian, Peoples R China
  • [ 13 ] [Hu, Fen]Fuzhou Univ, Coll Chem, Fuzhou 350108, Fujian, Peoples R China
  • [ 14 ] [Lan, Senchen]Fujian Agr & Forestry Univ, Coll Resources & Environm, Fujian Prov Key Lab Soil Environm Hlth & Regulat, Fuzhou 350002, Fujian, Peoples R China
  • [ 15 ] [Ci, Suqin]Fujian Agr & Forestry Univ, Coll Resources & Environm, Fujian Prov Key Lab Soil Environm Hlth & Regulat, Fuzhou 350002, Fujian, Peoples R China
  • [ 16 ] [Chen, Kai]Univ Chinese Acad Sci, Beijing 100049, Peoples R China
  • [ 17 ] [Lu, Zhiwen]Univ Chinese Acad Sci, Beijing 100049, Peoples R China
  • [ 18 ] [Gao, Jiyuan]Univ Chinese Acad Sci, Beijing 100049, Peoples R China
  • [ 19 ] [Wen, Zhenhai]Univ Chinese Acad Sci, Beijing 100049, Peoples R China

Reprint 's Address:

  • [Chen, Junxiang]Chinese Acad Sci, State Key Lab Struct Chem, Fuzhou 350002, Fujian, Peoples R China;;[Wen, Zhenhai]Chinese Acad Sci, State Key Lab Struct Chem, Fuzhou 350002, Fujian, Peoples R China;;[Chen, Junxiang]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Mat & Tech Hydrogen Energy, Fuzhou 350002, Fujian, Peoples R China;;[Wen, Zhenhai]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Prov Key Lab Mat & Tech Hydrogen Energy, Fuzhou 350002, Fujian, Peoples R China;;[Ci, Suqin]Fujian Agr & Forestry Univ, Coll Resources & Environm, Fujian Prov Key Lab Soil Environm Hlth & Regulat, Fuzhou 350002, Fujian, Peoples R China;;[Wen, Zhenhai]Univ Chinese Acad Sci, Beijing 100049, Peoples R China

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Source :

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION

Year: 2025

1 6 . 1 0 0

JCR@2023

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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