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author:

Lv, C. (Lv, C..) [1] | Liu, L.-P. (Liu, L.-P..) [2] | He, J.-H. (He, J.-H..) [3] | Yang, L. (Yang, L..) [4] | Liu, J.-T. (Liu, J.-T..) [5] | Xia, C.-Q. (Xia, C.-Q..) [6] | Huang, X.-Y. (Huang, X.-Y..) [7] | Feng, M.-L. (Feng, M.-L..) [8]

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Scopus

Abstract:

Due to the strong chemical toxicity and radiological hazard, uranium poses long-term threat to both environment and living organisms. However, soluble UO22+ ions with the mobility leads to difficulties in effectively capturing uranium from complex radioactive wastewater. Herein, the efficient U(VI) adsorption is achieved by MQ2-collagen fibers (MoS2-CF; M = Mo, W; Q = S, Se) composite prepared via co-ball milling MQ2 and CF, which exhibit higher uranium adsorption performance with the saturated adsorption capacity (q e) of 301 mg g−1 than pristine MQ2 due to their better hydrophilicity and the advantage of fibrous structure for better UO22+ transfer. The adsorption mechanism is revealed to be the synergistic interaction of abundant S2− sites from MoS2 and amino and carboxyl groups from CF towards UO22+. This work proposes a universal preparation method for low-cost and eco-friendly composite materials combining transition metal dichalcogenide with CF by co-ball milling for efficient uranium adsorption. © 2024 The Author(s).

Keyword:

adsorption collagen fiber composite material transition metal dichalcogenide uranium

Community:

  • [ 1 ] [Lv C.]College of Chemistry, Sichuan University, Chengdu, 610064, China
  • [ 2 ] [Lv C.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350002, China
  • [ 3 ] [Liu L.-P.]College of Intelligent Terminal Industry, Chengdu Technological University, Yibin, 644002, China
  • [ 4 ] [He J.-H.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350002, China
  • [ 5 ] [He J.-H.]College of Chemistry, Fuzhou University, Fuzhou, 350116, China
  • [ 6 ] [Yang L.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350002, China
  • [ 7 ] [Yang L.]College of Chemistry, Fuzhou University, Fuzhou, 350116, China
  • [ 8 ] [Liu J.-T.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350002, China
  • [ 9 ] [Liu J.-T.]College of Chemistry, Fuzhou University, Fuzhou, 350116, China
  • [ 10 ] [Xia C.-Q.]College of Chemistry, Sichuan University, Chengdu, 610064, China
  • [ 11 ] [Huang X.-Y.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350002, China
  • [ 12 ] [Huang X.-Y.]Fujian Province Joint Innovation Key Laboratory of Fuel and Materials in Clean Nuclear Energy System, Fujian Institute of Research on the Structure of Matter, Chinese Academy Sciences, Fuzhou, 350002, China
  • [ 13 ] [Feng M.-L.]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou, 350002, China
  • [ 14 ] [Feng M.-L.]Fujian Province Joint Innovation Key Laboratory of Fuel and Materials in Clean Nuclear Energy System, Fujian Institute of Research on the Structure of Matter, Chinese Academy Sciences, Fuzhou, 350002, China

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Source :

National Science Open

ISSN: 2097-1168

Year: 2025

Issue: 1

Volume: 4

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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