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author：

Dong, J. (Dong, J..) [1] | Gao, Q. (Gao, Q..) [2] | Wu, L. (Wu, L..) [3] | Yang, J. (Yang, J..) [4] | Liu, H. (Liu, H..) [5] | Wang, W. (Wang, W..) [6] | Tang, R. (Tang, R..) [7] | Li, J. (Li, J..) [8] | Cao, Z. (Cao, Z..) [9] | Liu, Y. (Liu, Y..) [10] | Xu, H. (Xu, H..) [11] | Zhang, P. (Zhang, P..) [12] | Meng, R. (Meng, R..) [13] | Xu, X. (Xu, X..) [15] | Zhang, Z. (Zhang, Z..) [16] | Li, T. (Li, T..) [17] | Chen, T. (Chen, T..) [18] | Liu, S. (Liu, S..) [19] | Zhang, Y. (Zhang, Y..) [20]

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Abstract：

Antimony　selenosulfide　(Sb2(S,Se)3)　solar　cells　suffer　from　charge　carrier　loss,　which　has　limited　the　power　conversion　efficiency　to　around　10%.　Here　we　develop　a　charge　carrier　management　strategy　using　a　textured　fluorine-doped　tin　oxide　substrate　as　the　front　contact　to　enhance　light　scattering　and　maximize　charge　generation.　To　overcome　voids　and　shunt　paths　introduced　by　the　textured　surface,　we　insert　a　SnO2　layer　by　atomic　layer　deposition　at　the　textured　fluorine-doped　tin　oxide/CdS　interface.　This　results　in　a　conformal　deposition　of　CdS　and　an　optimal　bandgap　profile　in　the　Sb2(S,Se)3　absorber,　which　improves　charge　transport　and　lowers　charge　recombination　at　the　interface　and　in　the　bulk,　respectively.　We　achieve　a　certified　efficiency　of　10.70%　sodium　selenosulfate-based　Sb2(S,Se)3　solar　cells　with　excellent　stability.　We　prove　the　generality　of　the　method　demonstrating　selenourea-based　Sb2(S,Se)3　and　upscaling　the　solar　cells　to　1　cm2.　The　results　represent　a　step　forward　in　the　development　of　antimony-based　solar　cells.　©　The　Author(s),　under　exclusive　licence　to　Springer　Nature　Limited　2025.

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  • [ 1 ] [Dong J.]Institute of Photoelectronic Thin Film Devices and Technology, State Key Laboratory of Photovoltaic Materials and Cells, Engineering Research Center of Thin Film Optoelectronics Technology, Ministry of Education, Nankai University, Tianjin, China
  • [ 2 ] [Gao Q.]Institute of Photoelectronic Thin Film Devices and Technology, State Key Laboratory of Photovoltaic Materials and Cells, Engineering Research Center of Thin Film Optoelectronics Technology, Ministry of Education, Nankai University, Tianjin, China
  • [ 3 ] [Wu L.]Key Laboratory of Weak-Light Nonlinear Photonics, Ministry of Education, School of Physics, Nankai University, Tianjin, China
  • [ 4 ] [Yang J.]Hefei National Research Center for Physical Science at the Microscale, Deep Space Exploration Laboratory, Department of Materials Science and Engineering, School of Chemistry and Materials Science, University of Science and Technology of China, Hefei, China
  • [ 5 ] [Liu H.]Institute of Photoelectronic Thin Film Devices and Technology, State Key Laboratory of Photovoltaic Materials and Cells, Engineering Research Center of Thin Film Optoelectronics Technology, Ministry of Education, Nankai University, Tianjin, China
  • [ 6 ] [Wang W.]Institute of Micronano Devices & Solar Cells, College of Physics & Information Engineering, Fuzhou University, Fuzhou, China
  • [ 7 ] [Tang R.]Hefei National Research Center for Physical Science at the Microscale, Deep Space Exploration Laboratory, Department of Materials Science and Engineering, School of Chemistry and Materials Science, University of Science and Technology of China, Hefei, China
  • [ 8 ] [Li J.]Hefei National Research Center for Physical Science at the Microscale, Deep Space Exploration Laboratory, Department of Materials Science and Engineering, School of Chemistry and Materials Science, University of Science and Technology of China, Hefei, China
  • [ 9 ] [Cao Z.]Institute of Photoelectronic Thin Film Devices and Technology, State Key Laboratory of Photovoltaic Materials and Cells, Engineering Research Center of Thin Film Optoelectronics Technology, Ministry of Education, Nankai University, Tianjin, China
  • [ 10 ] [Liu Y.]Institute of Photoelectronic Thin Film Devices and Technology, State Key Laboratory of Photovoltaic Materials and Cells, Engineering Research Center of Thin Film Optoelectronics Technology, Ministry of Education, Nankai University, Tianjin, China
  • [ 11 ] [Xu H.]Institute of Photoelectronic Thin Film Devices and Technology, State Key Laboratory of Photovoltaic Materials and Cells, Engineering Research Center of Thin Film Optoelectronics Technology, Ministry of Education, Nankai University, Tianjin, China
  • [ 12 ] [Zhang P.]Key Laboratory of Weak-Light Nonlinear Photonics, Ministry of Education, School of Physics, Nankai University, Tianjin, China
  • [ 13 ] [Meng R.]Institute of Photoelectronic Thin Film Devices and Technology, State Key Laboratory of Photovoltaic Materials and Cells, Engineering Research Center of Thin Film Optoelectronics Technology, Ministry of Education, Nankai University, Tianjin, China
  • [ 14 ] [Li J.]Institute of Photoelectronic Thin Film Devices and Technology, State Key Laboratory of Photovoltaic Materials and Cells, Engineering Research Center of Thin Film Optoelectronics Technology, Ministry of Education, Nankai University, Tianjin, China
  • [ 15 ] [Xu X.]Institute of Photoelectronic Thin Film Devices and Technology, State Key Laboratory of Photovoltaic Materials and Cells, Engineering Research Center of Thin Film Optoelectronics Technology, Ministry of Education, Nankai University, Tianjin, China
  • [ 16 ] [Zhang Z.]Institute of Photoelectronic Thin Film Devices and Technology, State Key Laboratory of Photovoltaic Materials and Cells, Engineering Research Center of Thin Film Optoelectronics Technology, Ministry of Education, Nankai University, Tianjin, China
  • [ 17 ] [Li T.]Institute of Photoelectronic Thin Film Devices and Technology, State Key Laboratory of Photovoltaic Materials and Cells, Engineering Research Center of Thin Film Optoelectronics Technology, Ministry of Education, Nankai University, Tianjin, China
  • [ 18 ] [Chen T.]Hefei National Research Center for Physical Science at the Microscale, Deep Space Exploration Laboratory, Department of Materials Science and Engineering, School of Chemistry and Materials Science, University of Science and Technology of China, Hefei, China
  • [ 19 ] [Liu S.]Dalian National Laboratory for Clean Energy, iChEM, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian, China
  • [ 20 ] [Zhang Y.]Institute of Photoelectronic Thin Film Devices and Technology, State Key Laboratory of Photovoltaic Materials and Cells, Engineering Research Center of Thin Film Optoelectronics Technology, Ministry of Education, Nankai University, Tianjin, China

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Nature Energy

ISSN： 2058-7546

Year： 2025

4 9 . 8 0 0

JCR@2023

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ESI Highly Cited Papers on the List： 0 Unfold All

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